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WSe/WS异质结构超晶格中莫尔激子的观测

Observation of moiré excitons in WSe/WS heterostructure superlattices.

作者信息

Jin Chenhao, Regan Emma C, Yan Aiming, Iqbal Bakti Utama M, Wang Danqing, Zhao Sihan, Qin Ying, Yang Sijie, Zheng Zhiren, Shi Shenyang, Watanabe Kenji, Taniguchi Takashi, Tongay Sefaattin, Zettl Alex, Wang Feng

机构信息

Department of Physics, University of California at Berkeley, Berkeley, CA, USA.

Graduate Group in Applied Science and Technology, University of California at Berkeley, Berkeley, CA, USA.

出版信息

Nature. 2019 Mar;567(7746):76-80. doi: 10.1038/s41586-019-0976-y. Epub 2019 Feb 25.

Abstract

Moiré superlattices enable the generation of new quantum phenomena in two-dimensional heterostructures, in which the interactions between the atomically thin layers qualitatively change the electronic band structure of the superlattice. For example, mini-Dirac points, tunable Mott insulator states and the Hofstadter butterfly pattern can emerge in different types of graphene/boron nitride moiré superlattices, whereas correlated insulating states and superconductivity have been reported in twisted bilayer graphene moiré superlattices. In addition to their pronounced effects on single-particle states, moiré superlattices have recently been predicted to host excited states such as moiré exciton bands. Here we report the observation of moiré superlattice exciton states in tungsten diselenide/tungsten disulfide (WSe/WS) heterostructures in which the layers are closely aligned. These moiré exciton states manifest as multiple emergent peaks around the original WSe A exciton resonance in the absorption spectra, and they exhibit gate dependences that are distinct from that of the A exciton in WSe monolayers and in WSe/WS heterostructures with large twist angles. These phenomena can be described by a theoretical model in which the periodic moiré potential is much stronger than the exciton kinetic energy and generates multiple flat exciton minibands. The moiré exciton bands provide an attractive platform from which to explore and control excited states of matter, such as topological excitons and a correlated exciton Hubbard model, in transition-metal dichalcogenides.

摘要

莫尔超晶格能够在二维异质结构中产生新的量子现象,其中原子薄层之间的相互作用定性地改变了超晶格的电子能带结构。例如,在不同类型的石墨烯/氮化硼莫尔超晶格中可以出现迷你狄拉克点、可调谐的莫特绝缘体态和霍夫施塔特蝴蝶图案,而在扭曲双层石墨烯莫尔超晶格中已经报道了关联绝缘态和超导性。除了对单粒子态有显著影响外,莫尔超晶格最近还被预测会存在诸如莫尔激子带等激发态。在这里,我们报告了在二硒化钨/二硫化钨(WSe₂/WS₂)异质结构中观察到的莫尔超晶格激子态,其中各层紧密对齐。这些莫尔激子态在吸收光谱中表现为围绕原始WSe₂ A激子共振的多个出现的峰,并且它们表现出与WSe₂单层以及大扭转角的WSe₂/WS₂异质结构中的A激子不同的栅极依赖性。这些现象可以用一个理论模型来描述,其中周期性的莫尔势比激子动能强得多,并产生多个平坦的激子微带。莫尔激子带提供了一个有吸引力的平台,可用于探索和控制过渡金属二卤化物中物质的激发态,如拓扑激子和关联激子哈伯德模型。

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