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在干燥-湿循环作用下,铀矿尾矿池压实土层的氡衰减特性。

Radon attenuation characteristics of compacted soil layer for uranium mill tailings pond subjected to drying-wetting cycles.

机构信息

School of Resources, Environmental and Safety Engineering, University of South China, Hengyang 421001, China.

School of Resources, Environmental and Safety Engineering, University of South China, Hengyang 421001, China; Hunan Province Engineering Technology Research Center of Uranium Tailings Treatment, University of South China, Hengyang 421001, China; Hunan Province Engineering Research Center of Radioactive Control Technology in Uranium Mining and Metallurgy, University of South China, Hengyang 421001, China.

出版信息

Sci Total Environ. 2022 Dec 10;851(Pt 2):158184. doi: 10.1016/j.scitotenv.2022.158184. Epub 2022 Aug 19.

Abstract

Compacted soil layer (CSL) is generally designed for uranium mill tailings (UMTs) pond to form the radon seals, whereas it is usually affected by drying-wetting environmental conditions. To summarize the radon attenuation degradation performance of CSL subjected to drying-wetting cycles, an experiment with the application of meteorological data was developed. This paper focuses on the evolution of the soil apparent porosity, soil integrity and radon attenuation characteristics of CSL during continuous drying-wetting cycles. Image processing and a nonmetal acoustic wave detector were applied to analyze variations in the soil surface and internal defects, and the radon concentration was measured to reveal the radon attenuation performance of the CSL. The results reveal that with successive drying-wetting cycles, the soil apparent porosity increased, and the soil pores were enlarged. The soil integrity underwent dynamic recombination or reorganization and eventually reached a steady state. Moreover, it was observed that the saturated state of the uppermost soil led to a sharp increase in radon concentration (capping effect), and the decrease in accumulated radon concentration during the initial period resulted from the coupling effect of soil moisture, temperature and ambient pressure. The observations confirm that the drying-wetting environmental conditions markedly affect the radon migration channels and environment in the CSL, which provides a theoretical foundation for UMTs pond governance and radiation safety management.

摘要

压实土壤层(CSL)通常用于铀矿尾矿(UMTs)池形成氡气密封,但它通常会受到干燥-湿润环境条件的影响。为了总结经历干燥-湿润循环的 CSL 的氡衰减降解性能,开发了一项应用气象数据的实验。本文重点研究了连续干燥-湿润循环过程中 CSL 的土壤表观孔隙率、土壤完整性和氡衰减特性的演变。图像处理和非金属声波探测器用于分析土壤表面和内部缺陷的变化,并测量氡浓度以揭示 CSL 的氡衰减性能。结果表明,随着干燥-湿润循环的进行,土壤表观孔隙率增加,土壤孔隙扩大。土壤完整性经历了动态重组或重新组合,最终达到稳定状态。此外,观察到最上层土壤的饱和状态导致氡浓度急剧增加(封顶效应),而在初期积累的氡浓度减少是由于土壤水分、温度和环境压力的耦合效应所致。这些观察结果证实,干燥-湿润环境条件显著影响 CSL 中的氡迁移通道和环境,为 UMTs 池治理和辐射安全管理提供了理论基础。

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