Behera Sudarshan, Balasubramanian Sundaram
Chemistry and Physics of Materials Unit, Jawaharlal Nehru Centre for Advanced Scientific Research, Bangalore 560 064, India.
Phys Chem Chem Phys. 2022 Sep 21;24(36):21904-21915. doi: 10.1039/d2cp02636h.
Proteins complexed electrostatically with polymer surfactants constitute a viscous liquid by themselves, called the solvent-free protein liquid (SFPL). A solution of SFPL in a room temperature ionic liquid (PS-IL) offers the protein hyperthermal stability, higher solubility and greater IL tolerance. A generic understanding of these protein-polymer systems is obtained herein through extensive atomistic molecular dynamics simulations of three different enzymes (lipase A, lysozyme and myoglobin) under various conditions. Along with increased intra-protein hydrogen bonding, the surfactant coating around the proteins imparts greater thermal stability, and also aids in screening protein-IL interactions, endowing them IL tolerance. The reduced surface polarity of the protein-polymer bioconjugate and hydrogen bonding between the ethylene glycol groups of the surfactant and the IL cation contribute to the facile solvation of the protein in its PS-IL form. The results presented here rationalize several experimental observations and will aid in the improved design of such hybrid materials for sustainable catalysis.
与聚合物表面活性剂通过静电作用复合的蛋白质自身构成一种粘性液体,称为无溶剂蛋白质液体(SFPL)。SFPL在室温离子液体(PS-IL)中的溶液赋予蛋白质超热稳定性、更高的溶解度和更大的离子液体耐受性。本文通过对三种不同酶(脂肪酶A、溶菌酶和肌红蛋白)在各种条件下进行广泛的原子分子动力学模拟,对这些蛋白质-聚合物体系有了一般性的认识。随着蛋白质内部氢键的增加,蛋白质周围的表面活性剂涂层赋予了更高的热稳定性,并且有助于屏蔽蛋白质与离子液体的相互作用,赋予它们离子液体耐受性。蛋白质-聚合物生物共轭物表面极性的降低以及表面活性剂的乙二醇基团与离子液体阳离子之间的氢键作用有助于蛋白质以其PS-IL形式的轻松溶剂化。这里给出的结果使几个实验观察结果合理化,并将有助于改进此类用于可持续催化的杂化材料的设计。