Wallace L A, Pellizzari E D, Hartwell T D, Sparacino C, Whitmore R, Sheldon L, Zelon H, Perritt R
Environ Res. 1987 Aug;43(2):290-307. doi: 10.1016/s0013-9351(87)80030-0.
EPA's TEAM Study has measured exposures to 20 volatile organic compounds in personal air, outdoor air, drinking water, and breath of approximately 400 residents of New Jersey, North Carolina, and North Dakota. All residents were selected by a probability sampling scheme to represent 128,000 inhabitants of Elizabeth and Bayonne, New Jersey, 131,000 residents of Greensboro, North Carolina, and 7000 residents of Devils Lake, North Dakota. Participants carried a personal monitor to collect two 12-hr air samples and gave a breath sample at the end of the day. Two consecutive 12-hr outdoor air samples were also collected on identical Tenax cartridges in the backyards of some of the participants. About 5000 samples were collected, of which 1500 were quality control samples. Ten compounds were often present in personal air and breath samples at all locations. Personal exposures were consistently higher than outdoor concentrations for these chemicals and were sometimes 10 times the outdoor concentrations. Indoor sources appeared to be responsible for much of the difference. Breath concentrations also often exceeded outdoor concentrations and correlated more strongly with personal exposures than with outdoor concentrations. Some activities (smoking, visiting dry cleaners or service stations) and occupations (chemical, paint, and plastics plants) were associated with significantly elevated exposures and breath levels for certain toxic chemicals. Homes with smokers had significantly increased benzene and styrene levels in indoor air. Residence near major point sources did not affect exposure.
美国环境保护局的“接触与微环境监测”(TEAM)研究测量了新泽西州、北卡罗来纳州和北达科他州约400名居民个人空气、室外空气、饮用水和呼出气体中20种挥发性有机化合物的接触情况。所有居民均通过概率抽样方案选取,以代表新泽西州伊丽莎白市和贝永市的12.8万居民、北卡罗来纳州格林斯伯勒市的13.1万居民以及北达科他州魔鬼湖市的7000名居民。参与者携带个人监测器收集两份12小时的空气样本,并在当天结束时提供一份呼出气体样本。还在一些参与者后院相同的Tenax采样管上收集了两份连续12小时的室外空气样本。共收集了约5000个样本,其中1500个是质量控制样本。在所有地点的个人空气和呼出气体样本中,经常能检测到10种化合物。这些化学物质的个人接触量始终高于室外浓度,有时是室外浓度的10倍。室内来源似乎是造成这种差异的主要原因。呼出气体浓度也经常超过室外浓度,并且与个人接触量的相关性比与室外浓度的相关性更强。一些活动(吸烟、光顾干洗店或服务站)和职业(化工、油漆和塑料厂)与某些有毒化学物质的接触量和呼出气体水平显著升高有关。有吸烟者的家庭室内空气中苯和苯乙烯水平显著增加。靠近主要点源的住所并未影响接触情况。