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微波对氮空位中心金刚石样品的加热效应。

Microwave Heating Effect on Diamond Samples of Nitrogen-Vacancy Centers.

作者信息

Wang Zheng, Zhang Jintao, Feng Xiaojuan, Xing Li

机构信息

Department of Precision Instrument, Tsinghua University, Beijing 100084, China.

National Institute of Metrology, Beijing 100029, China.

出版信息

ACS Omega. 2022 Aug 24;7(35):31538-31543. doi: 10.1021/acsomega.2c04232. eCollection 2022 Sep 6.

Abstract

Diamond samples of defects with negatively charged nitrogen-vacancy (NV) centers are promising solid-state spin sensors suitable for quantum information processing and highly sensitive measurements of magnetic, electric, and thermal fields at the nanoscale. A diamond defect with an NV center is unique for its robust temperature-dependent zero-field splitting of the triplet ground state. This property enables the optical readout of electron spin states through manipulation of the ground triplet state using microwave resonance with from 100 K to approximately 600 K. Thus, prohibiting from external thermal disturbances is crucial for an accurate measurement using NV-diamond sensors. Nevertheless, the external microwave field probably exerts a heating effect on the diamond sample of NV centers. To our knowledge, the microwave heating effect on the diamond samples of NV centers has yet to be quantitatively and systematically addressed. Our observation demonstrates the existence of a prominent microwave heating effect on the diamond samples of NV centers with the microwave irradiation in a continuous mode and some pulse sequence modes. The zero-field splitting is largely red-shifted by the temperature rises of the diamond samples. The effect will inevitably cause NV-diamond sensors to misread the true temperature of the target and disturb magnetic field detection by perturbing the spin precession of NV centers. Our observation demonstrates that such a phenomenon is negligible for the quantum lock-in XY8-N method.

摘要

具有带负电荷氮空位(NV)中心缺陷的金刚石样品是很有前景的固态自旋传感器,适用于量子信息处理以及对纳米尺度的磁场、电场和热场进行高灵敏度测量。具有NV中心的金刚石缺陷因其三重基态强大的与温度相关的零场分裂而独具特色。这一特性使得通过在100 K至约600 K的温度范围内利用微波共振操纵基态三重态来实现电子自旋态的光学读出。因此,对于使用NV金刚石传感器进行精确测量而言,防止受到外部热干扰至关重要。然而,外部微波场可能会对NV中心的金刚石样品产生加热效应。据我们所知,微波对NV中心金刚石样品的加热效应尚未得到定量和系统的研究。我们的观察表明,在连续模式和某些脉冲序列模式下,微波辐照会对NV中心的金刚石样品产生显著的微波加热效应。金刚石样品的温度升高会使零场分裂发生很大程度的红移。这种效应将不可避免地导致NV金刚石传感器误读目标的真实温度,并通过干扰NV中心的自旋进动来扰乱磁场检测。我们的观察表明,对于量子锁定XY8 - N方法而言,这种现象可以忽略不计。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/35f7/9453975/98be6400317e/ao2c04232_0002.jpg

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