Becerril David, Vázquez Omar, Piccotti Diego, Sandoval Elizabeth Mendoza, Cesca Tiziana, Mattei Giovanni, Noguez Cecilia, Pirruccio Giuseppe
Instituto de Física, Universidad Nacional Autónoma de México Apartado Postal 20-364 México D.F. 01000 Mexico
Department of Physics and Astronomy, University of Padova Via Marzolo 8 I-35131 Padova Italy.
Nanoscale Adv. 2020 Feb 11;2(3):1261-1268. doi: 10.1039/d0na00095g. eCollection 2020 Mar 17.
Honeycomb plasmonic lattices are paradigmatic examples of non-Bravais lattices. We experimentally measure surface lattice resonances in effectively free-standing honeycomb lattices composed of silver nanospheres. By combining numerical simulations with analytical methods, we analyze the dispersion relation and the near-field properties of these modes along high symmetry trajectories. We find that our results can be interpreted in terms of dipole-only interactions between the two non-equivalent triangular sublattices, which naturally lead to an asymmetric near-field distribution around the nanospheres. We generalize the interaction between the two sublattices to the case of variable adjacent interparticle distance within the unit cell, highlighting symmetry changes and diffraction degeneracy lifting associated to the transition between Bravais and non-Bravais lattices.
蜂窝状等离子体晶格是非布拉菲晶格的典型例子。我们通过实验测量了由银纳米球组成的有效独立蜂窝状晶格中的表面晶格共振。通过将数值模拟与分析方法相结合,我们沿着高对称轨迹分析了这些模式的色散关系和近场特性。我们发现,我们的结果可以用两个不等价三角形子晶格之间仅偶极相互作用来解释,这自然导致纳米球周围近场分布不对称。我们将两个子晶格之间的相互作用推广到晶胞内可变相邻粒子间距离的情况,突出了与布拉菲晶格和非布拉菲晶格之间转变相关的对称性变化和衍射简并解除。