Ding Chao, Gao Han, Geng Wenhui, Zhao Mingwen
School of Physics, State Key Laboratory of Crystal Materials, Shandong University Jinan 250100 Shandong China
Nanoscale Adv. 2020 Dec 26;3(4):1127-1135. doi: 10.1039/d0na00759e. eCollection 2021 Feb 23.
Plasmons in two-dimensional (2D) Dirac materials feature an interesting regime with a tunable frequency, and long propagating length and lifetime, but are rarely achieved in the visible light regime. Using a tight-binding (TB) model in combination with first-principles calculations, we investigated plasmon modes in a 2D Lieb lattice with a Dirac nodal-line electronic structure. In contrast to conventional 2D plasmons, anomalous plasmons in the Lieb lattice exhibit the unique features of a carrier-density-independent frequency, being Landau-damping free in a wide-range of wave vectors, a high frequency, and high subwavelength confinement. Remarkably, by using first-principles calculations, we proposed a candidate material, 2D BeC monolayer, to achieve these interesting plasmon properties. The plasmons in the BeC monolayer can survive up to the visible frequency region and propagate to large momentum transfer that has rarely been reported. The anomalous plasmons revealed in the Lieb lattice offer a promising platform for the study of 2D plasmons as well as the design of 2D plasmonic materials.
二维(2D)狄拉克材料中的等离激元具有频率可调、传播长度长和寿命长等有趣特性,但在可见光范围内却很少能实现。我们结合紧束缚(TB)模型和第一性原理计算,研究了具有狄拉克节线电子结构的二维Lieb晶格中的等离激元模式。与传统二维等离激元不同,Lieb晶格中的反常等离激元具有与载流子密度无关的频率、在很宽的波矢范围内无朗道阻尼、高频以及高亚波长限制等独特特性。值得注意的是,通过第一性原理计算,我们提出了一种候选材料——二维BeC单层,以实现这些有趣的等离激元特性。BeC单层中的等离激元能够在可见光频率区域内存在,并传播到很少有报道的大动量转移处。Lieb晶格中揭示的反常等离激元为二维等离激元的研究以及二维等离激元材料的设计提供了一个很有前景的平台。