Hunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, Changsha, 410083, P. R. China.
The State Key Laboratory of High Performance and Complex Manufacturing, College of Mechanical and Electrical Engineering, Central South University, Changsha, 410083, P. R. China.
Adv Sci (Weinh). 2022 Dec;9(34):e2204891. doi: 10.1002/advs.202204891. Epub 2022 Oct 17.
Directional water self-transport plays a crucial role in diverse applications such as biosensing and water harvesting. Despite extensive progress, current strategies for directional water self-transport are restricted to a short self-driving distance, single function, and complicated fabrication methods. Here, a lubricant-infused heterogeneous superwettability surface (LIHSS) for directional water self-transport is proposed on polyimide (PI) film through femtosecond laser direct writing and lubricant infusion. By tuning the parameters of the femtosecond laser, the wettability of PI film can be transformed into superhydrophobic or superhydrophilic. After trapping water droplets on the superhydrophilic surface and depositing excess lubricant, the asymmetrical wetting ridge drives water droplets by an attractive capillary force on the LIHSS. Notably, the maximum droplet self-driving distance can approach ≈3 mm, which is nearly twice as long as the previously reported strategies for direction water self-transport. Significantly, it is demonstrated that this strategy makes it possible to achieve water self-transport, anti-gravity pumping, and chemical microreaction on a tilted LIHSS. This work provides an efficient method to fabricate a promising platform for realizing directional water self-transport.
定向水自传输在生物传感和水收集等多种应用中起着至关重要的作用。尽管已经取得了广泛的进展,但目前用于定向水自传输的策略仅限于短距离的自主驱动、单一功能和复杂的制造方法。在这里,通过飞秒激光直写和润湿性处理,在聚酰亚胺(PI)薄膜上提出了一种用于定向水自传输的基于润滑剂的非均匀超润湿表面(LIHSS)。通过调整飞秒激光的参数,可以将 PI 薄膜的润湿性转变为超亲水或超疏水。在超亲水表面上捕获水滴并沉积多余的润滑剂后,不对称润湿脊通过在 LIHSS 上的吸引力毛细力驱动水滴。值得注意的是,最大液滴自驱动距离可接近≈3mm,几乎是先前报道的定向水自传输策略的两倍。重要的是,该策略能够在倾斜的 LIHSS 上实现水的自传输、反重力泵送和化学微反应。这项工作提供了一种高效的方法来制造一种很有前途的实现定向水自传输的平台。