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电子-反铁磁磁振子耦合诱导的强能带重整化和新兴铁磁性

Strong band renormalization and emergent ferromagnetism induced by electron-antiferromagnetic-magnon coupling.

作者信息

Yu T L, Xu M, Yang W T, Song Y H, Wen C H P, Yao Q, Lou X, Zhang T, Li W, Wei X Y, Bao J K, Cao G H, Dudin P, Denlinger J D, Strocov V N, Peng R, Xu H C, Feng D L

机构信息

Laboratory of Advanced Materials, State Key Laboratory of Surface Physics and Department of Physics, Fudan University, 200438, Shanghai, P. R. China.

Shanghai Research Center for Quantum Sciences, 201315, Shanghai, P. R. China.

出版信息

Nat Commun. 2022 Nov 2;13(1):6560. doi: 10.1038/s41467-022-34254-0.

DOI:10.1038/s41467-022-34254-0
PMID:36323685
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9630309/
Abstract

The interactions between electrons and antiferromagnetic magnons (AFMMs) are important for a large class of correlated materials. For example, they are the most plausible pairing glues in high-temperature superconductors, such as cuprates and iron-based superconductors. However, unlike electron-phonon interactions (EPIs), clear-cut observations regarding how electron-AFMM interactions (EAIs) affect the band structure are still lacking. Consequently, critical information on the EAIs, such as its strength and doping dependence, remains elusive. Here we directly observe that EAIs induce a kink structure in the band dispersion of BaKMnAs, and subsequently unveil several key characteristics of EAIs. We found that the coupling constant of EAIs can be as large as 5.4, and it shows strong doping dependence and temperature dependence, all in stark contrast to the behaviors of EPIs. The colossal renormalization of electron bands by EAIs enhances the density of states at Fermi energy, which is likely driving the emergent ferromagnetic state in BaKMnAs through a Stoner-like mechanism with mixed itinerant-local character. Our results expand the current knowledge of EAIs, which may facilitate the further understanding of many correlated materials where EAIs play a critical role.

摘要

电子与反铁磁磁振子(AFMMs)之间的相互作用对于一大类关联材料来说至关重要。例如,它们是高温超导体(如铜酸盐和铁基超导体)中最有可能的配对粘合剂。然而,与电子 - 声子相互作用(EPI)不同,关于电子 - AFMM相互作用(EAI)如何影响能带结构,仍缺乏明确的观测结果。因此,关于EAI的关键信息,如其强度和掺杂依赖性,仍然难以捉摸。在此,我们直接观测到EAI在BaKMnAs的能带色散中诱导出一个扭结结构,随后揭示了EAI的几个关键特征。我们发现,EAI的耦合常数可达5.4,并且它表现出强烈的掺杂依赖性和温度依赖性,这与EPI的行为形成鲜明对比。EAI对电子能带的巨大重整化增强了费米能处的态密度,这可能通过具有混合巡游 - 局域特性的类似斯托纳机制推动BaKMnAs中出现铁磁态。我们的结果扩展了当前对EAI的认识,这可能有助于进一步理解许多EAI在其中起关键作用的关联材料。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/60ca6d3f6818/41467_2022_34254_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/e5fb95e1b7d0/41467_2022_34254_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/44191d983e8c/41467_2022_34254_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/89372c46bd16/41467_2022_34254_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/6327d3685cf5/41467_2022_34254_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/60ca6d3f6818/41467_2022_34254_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/e5fb95e1b7d0/41467_2022_34254_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/44191d983e8c/41467_2022_34254_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/89372c46bd16/41467_2022_34254_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/6327d3685cf5/41467_2022_34254_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/10cf/9630309/60ca6d3f6818/41467_2022_34254_Fig5_HTML.jpg

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