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通过直流磁弛豫和交流多频磁化率研究确定高性能CaKFeAs超导体中的钉扎势

Pinning potential in highly performant CaKFeAs superconductor from DC magnetic relaxation and AC multi-frequency susceptibility studies.

作者信息

Ionescu A M, Ivan I, Crisan D N, Galluzzi A, Polichetti M, Ishida S, Iyo A, Eisaki H, Crisan A

机构信息

National Institute of Materials Physics, 405A Atomistilor Str., 077125, Magurele, Romania.

Department of Physics "E.R. Caianiello", University of Salerno, Via Giovanni Paolo II, 132, 84084Fisciano, Italy.

出版信息

Sci Rep. 2022 Nov 9;12(1):19132. doi: 10.1038/s41598-022-23879-2.

Abstract

We have investigated the pinning potential of high-quality single crystals of superconducting material CaKFeAs having high critical current density and very high upper critical field using both magnetization relaxation measurements and frequency-dependent AC susceptibility. Preliminary studies of the superconducting transition and of the isothermal magnetization loops confirmed the high quality of the samples, while temperature dependence of the AC susceptibility in high magnetic fields show absolutely no dependence on the cooling conditions, hence, no magnetic history. From magnetization relaxation measurements were extracted the values of the normalized pinning potential U*, which reveals a clear crossover between elastic creep and plastic creep. The extremely high values of U*, up to 1200 K around the temperature of 20 K lead to a nearly zero value of the probability of thermally-activated flux jumps at temperatures of interest for high-field applications. The values of the creep exponents in the two creep regimes resulted from the analysis of the magnetization relaxation data are in complete agreement with theoretical models. Pinning potentials were also estimated, near the critical temperature, from AC susceptibility measurements, their values being close to those resulted (at the same temperature and DC field) from the magnetization relaxation data.

摘要

我们使用磁化弛豫测量和频率相关的交流磁化率,研究了具有高临界电流密度和非常高的上临界场的超导材料CaKFeAs高质量单晶的钉扎势。对超导转变和等温磁化回线的初步研究证实了样品的高质量,而高磁场中交流磁化率的温度依赖性表明其完全不依赖于冷却条件,因此也不存在磁历史。从磁化弛豫测量中提取了归一化钉扎势U的值,该值揭示了弹性蠕变和塑性蠕变之间的明显转变。在20 K左右的温度下,U的值极高,高达1200 K,这导致在高场应用感兴趣的温度下热激活磁通跳跃的概率几乎为零。通过对磁化弛豫数据的分析得出的两种蠕变机制下的蠕变指数值与理论模型完全一致。在临界温度附近,还通过交流磁化率测量估计了钉扎势,其值与(在相同温度和直流场下)磁化弛豫数据得出的值接近。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7ecb/9646758/cda43156501c/41598_2022_23879_Fig1_HTML.jpg

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