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旋转圆盘动态过滤过程中聚丙烯酰胺/二氧化硅纳米复合材料改性水基钻井液的水动力分析及滤饼侵蚀特性

Hydrodynamic Analysis and Cake Erosion Properties of a Modified Water-Based Drilling Fluid by a Polyacrylamide/Silica Nanocomposite during Rotating-Disk Dynamic Filtration.

作者信息

Movahedi Hamed, Jamshidi Saeid, Hajipour Mastaneh

机构信息

Department of Chemical and Petroleum Engineering, Sharif University of Technology, Tehran11365-11155, Iran.

Department of Petroleum Engineering, Science and Research Branch, Islamic Azad University, Tehran14778-93855, Iran.

出版信息

ACS Omega. 2022 Nov 17;7(48):44223-44240. doi: 10.1021/acsomega.2c05688. eCollection 2022 Dec 6.

Abstract

In this study, the potential of using a polyacrylamide-silica nanocomposite (PAM-S) to control the filtration properties of bentonite water-based drilling muds under different salinity conditions was evaluated. Static filtration tests under low-pressure/low-temperature (LPLT) conditions accompanied by rheological measurements have been carried out to analyze the role of silica nanoparticles (NPs) and nanocomposites (NCs) in the base fluid properties. Moreover, high-pressure/high-temperature (HPHT) static filtration was also investigated to evaluate the thermal stability of PAM-S. Afterward, dynamic filtration has been conducted in a filtration cell equipped with an agitating system with a disk-type impeller to investigate the hydrodynamic and formation of a filter cake under shear flow conditions. Fluid flow velocity and wall shear stress (WSS) distribution over the filter cake were analyzed using an exact 3D computational fluid dynamic (CFD) simulation. A transparent filtration cell with a camera was used to accurately record the fluid flow field inside the filter press and validate the CFD results. The obtained results indicated that adding silica NPs at a concentration of less than 2 wt % increases the fluid loss due to reducing rheological properties such as yield point. While silica NPs could not significantly change the mud properties, the experimental results showed that, under both LPLT and HPHT conditions, the PAM-S NC could reduce the total filtration loss by 70% at a low concentration of 0.75 wt %. Moreover, during dynamic filtration, the results indicated that there is a linear relationship between the cake thickness and the inverse of WSS at different operating pressures. However, no correlation could be found between predeposited mud cake erosion and WSS. At a rotating disk speed of 1000 rpm, more than 60% of the predeposited mud cake was eroded after 30 min for a saline mud sample while for the NC-treated mud sample cake erosion is considerably reduced and reaches up to 20% at 1.5 wt % PAM-S.

摘要

在本研究中,评估了使用聚丙烯酰胺-二氧化硅纳米复合材料(PAM-S)在不同盐度条件下控制膨润土水基钻井液过滤性能的潜力。进行了低压/低温(LPLT)条件下的静态过滤试验并伴有流变学测量,以分析二氧化硅纳米颗粒(NPs)和纳米复合材料(NCs)在基液性能中的作用。此外,还研究了高压/高温(HPHT)静态过滤以评估PAM-S的热稳定性。随后,在配备有盘式叶轮搅拌系统的过滤池中进行了动态过滤,以研究剪切流条件下的流体动力学和滤饼形成。使用精确的三维计算流体动力学(CFD)模拟分析了滤饼上的流体流速和壁面剪应力(WSS)分布。使用带有摄像头的透明过滤池准确记录压滤机内部的流体流场并验证CFD结果。所得结果表明,添加浓度低于2 wt%的二氧化硅NPs会因降低诸如屈服点等流变性能而增加滤失量。虽然二氧化硅NPs不会显著改变泥浆性能,但实验结果表明,在LPLT和HPHT条件下,PAM-S NC在0.75 wt%的低浓度下可将总滤失量降低70%。此外,在动态过滤过程中,结果表明在不同操作压力下滤饼厚度与WSS的倒数之间存在线性关系。然而,在预沉积泥饼侵蚀与WSS之间未发现相关性。在1000 rpm的转盘速度下,对于含盐泥浆样品,30分钟后超过60%的预沉积泥饼被侵蚀,而对于经NC处理的泥浆样品,在1.5 wt%的PAM-S下泥饼侵蚀显著减少,达到20%。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4617/9730759/50f421966e9a/ao2c05688_0002.jpg

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