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基于多种吸收机制协同效应的宽带太阳能吸收等离子体纳米结构

Plasmonic Nanostructures for Broadband Solar Absorption Based on Synergistic Effect of Multiple Absorption Mechanisms.

作者信息

Su Junli, Liu Dingquan, Sun Leihao, Chen Gang, Ma Chong, Zhang Qiuyu, Li Xingyu

机构信息

Shanghai Institute of Technical Physics, Chinese Academy of Sciences, Shanghai 200083, China.

School of Physical Science and Technology, ShanghaiTech University, Shanghai 200031, China.

出版信息

Nanomaterials (Basel). 2022 Dec 15;12(24):4456. doi: 10.3390/nano12244456.

Abstract

The growing attention to solar energy has motivated the development of highly efficient solar absorbers. In this study, a high-performance meta-structure solar absorber (MSSA) based on a tungsten truncated cone structure combined with a film resonator structure has been proposed and demonstrated numerically. The designed structure exhibits over 97.1% total solar absorption efficiency and less than 8.5% total thermal emissivity under the condition of one solar concentration, hence reaching 91.6% photothermal conversion efficiency at 100 °C. In addition, the proposed MSSA achieves promisingly high spectrum absorptance of over 97.8% in the ultraviolet, visible and near-infrared regions (280-1700 nm). Based on the simulation analysis, the enhanced light absorption is attributed to the synergistic effect of the magnetic polaritons (MPs) on the nanostructured metal surface, the cavity plasmon resonance between the truncated cones that can form light-trapping structures, the magnetic field resonance of the metal-insulator-metal (MIM) optical resonator and the inherent loss of tungsten. The impedance of the absorber is well matched with free space. Furthermore, the optimized absorber shows great potential in solar thermophotovoltaic applications that require wide-angle polarization-independent ultra-broadband light response characteristics.

摘要

对太阳能日益增长的关注推动了高效太阳能吸收器的发展。在本研究中,基于钨截锥结构与薄膜谐振器结构相结合的高性能超材料结构太阳能吸收器(MSSA)已被提出并进行了数值验证。所设计的结构在一个太阳聚光条件下展现出超过97.1%的总太阳能吸收效率和低于8.5%的总热发射率,因此在100℃时达到91.6%的光热转换效率。此外,所提出的MSSA在紫外、可见和近红外区域(280 - 1700nm)实现了超过97.8%的高光谱吸收率。基于模拟分析,增强的光吸收归因于纳米结构金属表面上磁极化子(MPs)的协同效应、可形成光捕获结构的截锥之间的腔等离子体共振、金属 - 绝缘体 - 金属(MIM)光学谐振器的磁共振以及钨的固有损耗。吸收器的阻抗与自由空间良好匹配。此外,优化后的吸收器在需要宽角度偏振无关超宽带光响应特性的太阳能热光伏应用中显示出巨大潜力。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/a4fc/9782161/5ad6e42dc94a/nanomaterials-12-04456-g001.jpg

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