Li Jiuhui, Wu Zhengfang, He Hongshi, Lu Wenxi
Key Laboratory of Geographical Processes and Ecological Security in Changbai Mountains, Ministry of Education, School of Geographical Sciences, Northeast Normal University, Changchun, 130022, China.
Key Laboratory of Groundwater Resources and Environment, Ministry of Education, Jilin University, Changchun, 130021, China.
Environ Sci Pollut Res Int. 2023 Mar;30(13):38663-38682. doi: 10.1007/s11356-022-24671-5. Epub 2022 Dec 30.
The simulation optimization method was used to the identification of light nonaqueous phase liquid (LNAPL) groundwater contamination source (GCS) with the help of a hypothetical case in this study. When applying the simulation optimization method to identify GCS, it was a common technical means to establish surrogate model for the simulation model to participate in the iterative calculation to reduce the calculation load and calculation time. However, it was difficult for a single modeling method to establish surrogate model with high accuracy for the LNAPL contamination multiphase flow simulation model (MFSM). To give full play to advantages of single surrogate model and improve the accuracy of the surrogate model to the MFSM, a combination of deep belief neural network (DBNN) and long short-term memory (LSTM) neural network was used to establish artificial intelligence ensemble surrogate model (AIESM) for the MFSM. At the same time, to reduce the influence of noise in observed concentrations on the accuracy of the identification results, empirical mode decomposition (EMD) and wavelet analysis methods were used to denoise the observed concentrations, and their noise reduction effects were compared. The observed concentrations with better noise reduction effect and the observed concentrations without denoising were used to construct the objective function, and constraints of the optimization model were determined meanwhile. Then, the objective function and the constraints were integrated to build the optimization model to identify GCS and simulation model parameters. Applying the AIESM instead of the MFSM to embed in the optimization model and participate in the iterative calculation. Finally, the genetic algorithm (GA) was used to solve the optimization model to obtain the identification results of GCS and simulation model parameters. The results showed that compared with the single DBNN and LSTM surrogate models, AIESM obtained the highest accuracy and could replace the MFSM to participate in the iterative calculation, thereby reducing the calculation load and calculation time by more than 99%. Comparing with the wavelet analysis, EMD could reduce the noise in the concentrations more effectively, improved the accuracy of the approximated concentrations to the actual values, and increased the accuracy of the GCSs identification results by 1.45%.
本研究借助一个假设案例,采用模拟优化方法来识别轻质非水相液体(LNAPL)地下水污染源(GCS)。在应用模拟优化方法识别GCS时,为降低计算量和计算时间,建立替代模型参与迭代计算是模拟模型常用的技术手段。然而,单一建模方法难以针对LNAPL污染多相流模拟模型(MFSM)建立高精度替代模型。为充分发挥单一替代模型的优势,提高替代模型对MFSM的精度,采用深度信念神经网络(DBNN)和长短期记忆(LSTM)神经网络相结合的方法,为MFSM建立人工智能集成替代模型(AIESM)。同时,为降低观测浓度中的噪声对识别结果精度的影响,采用经验模态分解(EMD)和小波分析方法对观测浓度进行去噪,并比较了它们的降噪效果。利用降噪效果较好的观测浓度和未去噪的观测浓度构建目标函数,同时确定优化模型的约束条件。然后,将目标函数和约束条件整合,构建用于识别GCS和模拟模型参数的优化模型。应用AIESM替代MFSM嵌入优化模型并参与迭代计算。最后,使用遗传算法(GA)求解优化模型,得到GCS和模拟模型参数的识别结果。结果表明,与单一的DBNN和LSTM替代模型相比,AIESM具有最高的精度,能够替代MFSM参与迭代计算,从而将计算量和计算时间减少99%以上。与小波分析相比,EMD能更有效地降低浓度中的噪声,提高近似浓度与实际值的精度,使GCS识别结果的精度提高1.45%。