Stuart G R, Chambers R W
Department of Biochemistry, Dalhousie University, Halifax, Nova Scotia, Canada.
Nucleic Acids Res. 1987 Sep 25;15(18):7451-62. doi: 10.1093/nar/15.18.7451.
A general synthesis of a deoxyoligonucleotide with an AP site at a preselected sequence is described. Deoxyuridine is introduced during routine oligonucleotide syntheses of d(TTTUTTTT) and d(AAAAGTTUAAAACAT). Treatment with uracil DNA-glycosylase produces d(TTTrTTTT), where r = deoxyribose, and d(AAAAGTTprpAAAACAT). KM and Vmax are: d(TTTUTTTT), 7.3 X 10(-9)M and 2.0 X 10(-9) mumol/min; d(AAAAGTTUAAAACAT), 1.5 X 10(-8) M and 6.4 X 10(-9) mumol/min. Both d(AAAAGTTprpAAAACAT) and d(TTTprpTTTT) undergo rapid beta-elimination in 1 M piperidine at 25 degrees giving two oligonucleotide fragments, d(AAAAGTTpr') and d(pAAAACAT), where r' = -O-CH2-CHOH-CH=CH-CHO (or its hemiacetal form). The fragment, d(AAAAGTTpr'), which can be isolated by reverse phase chromatography, is resistant to the 3'----5' exonuclease activity of snake venom phosphodiesterase. Endonucleolytic hydrolysis of the penultimate phosphodiester occurs removing pTpr' and generating a normal 3'-OH end. In 1 M piperidine at 90 degrees two beta-eliminations occur producing the oligonucleotides d(AAAAGTTp) and d(pAAAACAT) from d(AAAAGTTprpAAAACAT); d(TTTp) and d(pTTTT) from d(TTTprpTTTT).
本文描述了一种在预选序列处带有脱嘌呤嘧啶(AP)位点的脱氧寡核苷酸的通用合成方法。在d(TTTUTTTT)和d(AAAAGTTUAAAACAT)的常规寡核苷酸合成过程中引入脱氧尿苷。用尿嘧啶DNA糖基化酶处理后分别产生d(TTTrTTTT)(其中r = 脱氧核糖)和d(AAAAGTTprpAAAACAT)。米氏常数(KM)和最大反应速度(Vmax)分别为:d(TTTUTTTT),7.3×10⁻⁹M和2.0×10⁻⁹μmol/min;d(AAAAGTTUAAAACAT),1.5×10⁻⁸M和6.4×10⁻⁹μmol/min。d(AAAAGTTprpAAAACAT)和d(TTTprpTTTT)在25℃的1M哌啶中都会迅速发生β-消除反应,生成两个寡核苷酸片段,d(AAAAGTTpr')和d(pAAAACAT),其中r' = -O-CH₂-CHOH-CH=CH-CHO(或其半缩醛形式)。片段d(AAAAGTTpr')可通过反相色谱法分离,它对蛇毒磷酸二酯酶的3'→5'外切核酸酶活性具有抗性。倒数第二个磷酸二酯键发生内切水解,去除pTpr'并产生正常的3'-OH末端。在90℃的1M哌啶中,d(AAAAGTTprpAAAACAT)会发生两次β-消除反应,生成寡核苷酸d(AAAAGTTp)和d(pAAAACAT);d(TTTprpTTTT)则生成d(TTTp)和d(pTTTT)。