Department of Physics, NC State University, Raleigh, NC 27695, United States of America.
Nanotechnology. 2023 Feb 15;34(18):185201. doi: 10.1088/1361-6528/acb443.
The transmission of light through sub-wavelength apertures (zero-mode waveguides, ZMW) in metal films is well-explored. It introduces both an amplitude modulation as well as a phase shift to the oscillating electromagnetic field. We propose a nanophotonic interferometer by bringing two ZMW (∼100 nm diameter) in proximity and monitoring the distribution of transmitted light in the back-focal plane of collecting microscope objective (1.3 N.A.). We demonstrate that both an asymmetry induced by the binding of a quantum dot in one of the two ZMW, as well as an asymmetry in ZMW diameter yield qualitatively similar transmission patterns. We find that the complex pattern can be quantified through a scalar measure of asymmetry along the symmetry axis of the aperture pair. In a combined experimental and computational exploration of detectors with differing ZMW diameters, we find that the scalar asymmetry is a monotonous function of the diameter difference of the two apertures, and that the scalar asymmetry measure is higher if the sample is slightly displaced from the focal plane of the collecting microscope objective. An optimization of the detector geometry determined that the maximum response is achieved at an aperture separation that is comparable to the wavelength on the exit side of the sensor. For small separations of apertures, on the order of a quarter of the wavelength and less, the signal is strongly polarization dependent, while for larger separations, on the order of the wavelength or larger, the signal becomes essentially polarization-independent.
光在金属薄膜中的亚波长孔径(零模波导,ZMW)中的传输已经得到了很好的研究。它会对振荡电磁场同时引入幅度调制和相位移动。我们通过将两个 ZMW(直径约为 100nm)放置得很近,并在收集显微镜物镜的后焦平面(1.3 N.A.)上监测传输光的分布,提出了一种纳米光子干涉仪。我们证明了一个 ZMW 中的量子点结合引起的不对称性,以及 ZMW 直径的不对称性,都会产生定性相似的传输模式。我们发现,通过对孔径对对称轴上的不对称性进行标量测量,可以对复杂的图案进行量化。在对具有不同 ZMW 直径的探测器进行实验和计算的综合探索中,我们发现,标量不对称性是两个孔径直径差的单调函数,如果样品稍微偏离收集显微镜物镜的焦平面,那么标量不对称性的测量值就会更高。对探测器几何形状的优化确定了在传感器出射侧的波长可比的孔径分离处可实现最大响应。对于孔径分离较小的情况,大约为四分之一波长或更小,信号强烈依赖于偏振,而对于较大的分离情况,大约为波长或更大,信号基本上与偏振无关。