Zhang Jinxi, Wu Chen, Zhang Qiankun, Liu Jing
State Key Laboratory of Precision Measurement Technology and Instrument, School of Precision Instruments and Opto-electronics Engineering, Tianjin University, No. 92 Weijin Road, Tianjin, 300072, People's Republic of China.
Key Laboratory of the Ministry of Education for Optoelectronic Measurement Technology and Instruments, Beijing Information Science and Technology University, Beijing 100192, People's Republic of China.
Nanotechnology. 2023 Feb 3;34(15). doi: 10.1088/1361-6528/acb447.
Two-dimensional (2D) materials are promising candidates for developing next generation electronic/optoelectronic devices with programmable multi functions, due to their widely tunable properties by various physical stimuli. Mechanical strain is one of the most promising means to effectively modulate the physical properties of 2D materials. Nevertheless, few studies reported micro/nano scale controllable strain application platforms, limiting the development of novel mechano-electrical/optoelectrical devices based on 2D materials. This work proposes surface acoustic wave (SAW) device as a controllable strain modulation platform for 2D materials with sub-micro scale resolution. The platform uses the piezoelectric material (LiNbO) as the substrate, which is deposited with interdigitated transducers (IDT) to generate SAW on the surface. The propagation of SAW causes surface deformation, which is then transferred to the 2D materials on the substrate. The period of the surface deformation/strain is related with that of SAW, which is determined by the period of IDT with nano meter scale. It is demonstrated that the photo luminescence spectrum of a 2D ReSflake on this platform gradually shifts with the SAW excitation power, which reaches a shift of 3 nm as the SAW excitation power achieves 26 dBm, corresponding to a band gap increase of 5 meV. Meanwhile, the platform is also capable to provide acousto-electric coupling between SAW and 2D materials, which is demonstrated by the shift of the SAW resonant frequency due to the re-distribution of photo-generated carriers in ReSupon light illumination.
二维(2D)材料因其可通过各种物理刺激实现广泛可调的特性,有望成为开发具有可编程多功能的下一代电子/光电器件的候选材料。机械应变是有效调制二维材料物理特性最具前景的手段之一。然而,很少有研究报道微纳尺度可控应变应用平台,这限制了基于二维材料的新型机电/光电器件的发展。这项工作提出将表面声波(SAW)器件作为一种具有亚微米尺度分辨率的二维材料可控应变调制平台。该平台使用压电材料(LiNbO)作为衬底,在其上沉积叉指换能器(IDT)以在表面产生SAW。SAW的传播会引起表面变形,然后传递到衬底上的二维材料。表面变形/应变的周期与SAW的周期相关,SAW的周期由具有纳米尺度的IDT的周期决定。结果表明,该平台上二维ReS薄片的光致发光光谱随SAW激发功率逐渐移动,当SAW激发功率达到26 dBm时,移动达到3 nm,对应带隙增加5 meV。同时,该平台还能够在SAW和二维材料之间提供声电耦合,这通过在光照下ReS中光生载流子重新分布导致SAW共振频率的移动得到证明。