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三维拓扑磁单极及其在铁磁亚晶格中的相互作用。

Three-dimensional topological magnetic monopoles and their interactions in a ferromagnetic meta-lattice.

机构信息

Department of Physics & Astronomy and California NanoSystems Institute, University of California, Los Angeles, Los Angeles, CA, USA.

STROBE Science and Technology Center, University of Colorado and NIST, Boulder, CO, USA.

出版信息

Nat Nanotechnol. 2023 Mar;18(3):227-232. doi: 10.1038/s41565-022-01311-0. Epub 2023 Jan 23.

Abstract

Topological magnetic monopoles (TMMs), also known as hedgehogs or Bloch points, are three-dimensional (3D) non-local spin textures that are robust to thermal and quantum fluctuations due to the topology protection. Although TMMs have been observed in skyrmion lattices, spinor Bose-Einstein condensates, chiral magnets, vortex rings and vortex cores, it has been difficult to directly measure the 3D magnetization vector field of TMMs and probe their interactions at the nanoscale. Here we report the creation of 138 stable TMMs at the specific sites of a ferromagnetic meta-lattice at room temperature. We further develop soft X-ray vector ptycho-tomography to determine the magnetization vector and emergent magnetic field of the TMMs with a 3D spatial resolution of 10 nm. This spatial resolution is comparable to the magnetic exchange length of transition metals, enabling us to probe monopole-monopole interactions. We find that the TMM and anti-TMM pairs are separated by 18.3 ± 1.6 nm, while the TMM and TMM, and anti-TMM and anti-TMM pairs are stabilized at comparatively longer distances of 36.1 ± 2.4 nm and 43.1 ± 2.0 nm, respectively. We also observe virtual TMMs created by magnetic voids in the meta-lattice. This work demonstrates that ferromagnetic meta-lattices could be used as a platform to create and investigate the interactions and dynamics of TMMs. Furthermore, we expect that soft X-ray vector ptycho-tomography can be broadly applied to quantitatively image 3D vector fields in magnetic and anisotropic materials at the nanoscale.

摘要

拓扑磁单极子(TMM),也称为刺猬或布洛赫点,是三维(3D)非局域自旋纹理,由于拓扑保护,它们对热和量子涨落具有鲁棒性。尽管 TMM 已在螺旋体晶格、自旋玻色-爱因斯坦凝聚体、手性磁体、涡旋环和涡旋核中被观察到,但很难直接测量 TMM 的三维磁化矢量场并在纳米尺度上探测它们的相互作用。在这里,我们报告了在室温下铁磁亚晶格的特定位置上创建了 138 个稳定的 TMM。我们进一步开发了软 X 射线矢量相衬层析成像技术,以确定 TMM 的磁化矢量和衍生磁场,具有 10nm 的 3D 空间分辨率。该空间分辨率与过渡金属的磁交换长度相当,使我们能够探测单极子-单极子相互作用。我们发现 TMM 和反 TMM 对之间的距离为 18.3±1.6nm,而 TMM 和 TMM、反 TMM 和反 TMM 对之间的距离分别稳定在较长的 36.1±2.4nm 和 43.1±2.0nm。我们还观察到亚晶格中的磁空洞产生的虚拟 TMM。这项工作表明,铁磁亚晶格可以用作创建和研究 TMM 相互作用和动力学的平台。此外,我们预计软 X 射线矢量相衬层析成像技术可以广泛应用于在纳米尺度上定量成像磁性和各向异性材料的 3D 矢量场。

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