Université de Lorraine, Institut Jean Lamour, UMR, 7198 CNRS, Nancy, France.
Nat Commun. 2023 Jan 27;14(1):445. doi: 10.1038/s41467-023-36164-1.
When exciting a magnetic material with a femtosecond laser pulse, the amplitude of magnetization is no longer constant and can decrease within a time scale comparable to the duration of the optical excitation. This ultrafast demagnetization can even trigger an ultrafast, out of equilibrium, phase transition to a paramagnetic state. The reciprocal effect, namely an ultrafast remagnetization from the zero magnetization state, is a necessary ingredient to achieve a complete ultrafast reversal. However, the speed of remagnetization is limited by the universal critical slowing down which appears close to a phase transition. Here we demonstrate that magnetization can be reversed in a few hundreds of femtoseconds by overcoming the critical slowing down thanks to ultrafast spin cooling and spin heating mechanisms. We foresee that these results outline the potential of ultrafast spintronics for future ultrafast and energy efficient magnetic memory and storage devices. Furthermore, this should motivate further theoretical works in the field of femtosecond magnetization reversal.
当用飞秒激光脉冲激发磁性材料时,磁化强度不再保持恒定,而是在与光激发持续时间可比的时间尺度内减小。这种超快退磁甚至可以引发超快、非平衡的顺磁态相变。相反的效果,即从零磁化强度状态的超快再磁化,是实现完全超快反转的必要条件。然而,再磁化的速度受到普遍的临界减速的限制,这种临界减速接近相变。在这里,我们通过超快自旋冷却和自旋加热机制克服临界减速,证明在几百飞秒内可以反转磁化。我们预计这些结果将为超快自旋电子学在未来超快和节能磁记忆和存储设备中的应用提供潜力。此外,这应该激励在飞秒磁化反转领域的进一步理论工作。