Department of Energy Systems Research, Ajou University, Suwon, 16499, Republic of Korea.
Department of Materials Science and Engineering, Ajou University, Suwon, 16499, Republic of Korea.
Adv Mater. 2023 May;35(18):e2210907. doi: 10.1002/adma.202210907. Epub 2023 Mar 19.
Light-intensity selective superlinear photodetectors with ultralow dark current can provide an essential breakthrough for the development of high-performing near-sensor vision processing. However, the development of near-sensor vision processing is not only conceptually important for device operation (given that sensors naturally exhibit linear/sublinear responses), but also essential to get rid of the massive amount of data generated during object sensing and classification with noisy inputs. Therefore, achieving the giant superlinear photoresponse while maintaining the picoampere leakage current, irrespective of the measurement bias, is one of the most challenging tasks. Here, Mott material (vanadium dioxide) and silicon-based integrated infrared photodetectors are developed that show giant superlinear photoresponse (exponent >18) and ultralow dark current of 4.46 pA. Specifically, the device demonstrates an electro-opto-coupled insulator-to-metal transition, which leads to outstanding photocurrent on/off ratio (>10 ), a high responsivity (>1 mA W ), and excellent detectivity (>10 Jones), while maintaining response speed (τ = 6 µs and τ = 10 µs). Further, intensity-selective near-sensor processing is demonstrated and night vision pattern reorganization even with noisy inputs is exhibited. This research will pave the way for the creation of high-performance photodetectors with potential uses, such as in night vision, pattern recognition, and neuromorphic processing.
具有超低暗电流的弱光选择超线性光电探测器可为高性能近传感器视觉处理的发展提供重要突破。然而,近传感器视觉处理的发展不仅在器件操作概念上很重要(因为传感器自然呈现线性/次线性响应),而且对于摆脱在嘈杂输入下进行物体感应和分类时产生的大量数据也至关重要。因此,在不考虑测量偏置的情况下,实现巨超线性光电响应同时保持皮安级泄漏电流是最具挑战性的任务之一。在这里,开发了基于莫特材料(二氧化钒)和硅的集成红外光电探测器,它们表现出巨大的超线性光电响应(指数>18)和超低的暗电流(4.46 pA)。具体而言,该器件表现出电光耦合的绝缘到金属转变,从而导致出色的光电电流开/关比(>10 )、高响应度(>1 mA W )和优异的探测率(>10 琼斯),同时保持响应速度(τ=6 μs 和 τ=10 μs)。此外,还展示了强度选择性的近传感器处理,甚至在嘈杂输入下也能实现夜视模式重组。这项研究将为创建具有潜在用途的高性能光电探测器铺平道路,例如在夜视、模式识别和神经形态处理方面。