Recent advances in bio-inspired ionic liquid-based interfacial materials from preparation to application.

Natural creatures always display unique and charming functions, such as the adhesion of mussels and the lubrication of Nepenthes, to maintain their life activities. Bio-inspired interfacial materials infused with liquid, especially for ionic liquids (ILs), have been designed and prepared to meet the emerging and rising needs of human beings. In this review, we first summarize the recent development of bio-inspired IL-based interfacial materials (BILIMs), ranging from the synthesis strategy to the design principle. Then, we discuss the advanced applications of BILIMs from anti-adhesive aspects (e.g., anti-biofouling, anti-liquid fouling, and anti-solid fouling) to adhesive aspects (e.g., biological sensor, adhesive tape, and wound dressing). Finally, the current limitations and future prospects of BILIMs are provided to feed the actual needs.