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[排放与气象条件对武汉新冠疫情封控期间各站点空气污染物的影响]

[Impacts of Emission and Meteorological Conditions on Air Pollutants at Various Sites Around the COVID-19 Lockdown in Wuhan].

作者信息

Xiong Jiang-He, Kong Shao-Fei, Zheng Huang, Xiao Wan, Liu Ao, Zhu Ming-Ming

机构信息

School of Environmental Studies, China University of Geosciences, Wuhan 430078, China.

Research Centre for Complex Air Pollution of Hubei Province, Wuhan 430078, China.

出版信息

Huan Jing Ke Xue. 2023 Feb 8;44(2):670-679. doi: 10.13227/j.hjkx.202203269.

Abstract

The random forest algorithm was used to separate the mass concentrations of six air pollutants (SO, NO, CO, PM, PM, and O) contributed by emissions and meteorological conditions. Their variations for five types of sites including Wuhan's central urban, suburb, industrial, the third ring road traffic, and urban background sites were investigated. The results showed that the values of PM/CO, PM/CO, and NO/CO during the lockdown period decreased by 10.8-21.7, 9.34-24.7, and 14.4-22.1 times compared with the period before the lockdown, indicating that the contributions of emissions to PM, PM, and NO were reduced. O/CO increased by 50.1-61.5 times, implying that the secondary formation increased obviously. The contributions of emissions to various types of pollutants all increased after the lockdown. During the lockdown period, affected by the operation of some uninterrupted industrial processes, PM concentrations in industrial areas dropped the least (20.5%). Compared with the lockdown period, residential activities, transportation, and industrial production were basically restored after the lockdown, resulting in the alleviation of the reduction in PM emission-related concentrations. The increase in emission-related O concentrations could be associated with the decreased NO and PM concentrations during the lockdown period. The elevated O partially offset the improved air quality brought by the reduced NOand PM concentrations. After the lockdown, (O) related with meteorology at the suburban and urban background sites increased by 16.2 μg·m and 16.1 μg·m, respectively, which could be attributed to the increased ambient temperature and decreased relative humidity. The decrease in PM and increase in O concentrations caused by reduced traffic and industrial emissions at the third ring road traffic and central urban regions can provide reference for the current coordinated and precise control of PM and O in subregions.

摘要

随机森林算法被用于区分由排放和气象条件导致的六种空气污染物(二氧化硫、氮氧化物、一氧化碳、细颗粒物、可吸入颗粒物和臭氧)的质量浓度。研究了武汉市中心城区、郊区、工业区、三环线交通区和城市背景区这五类站点的污染物浓度变化情况。结果表明,封控期间细颗粒物与一氧化碳、可吸入颗粒物与一氧化碳、氮氧化物与一氧化碳的比值相较于封控前分别下降了10.8至21.7倍、9.34至24.7倍和14.4至22.1倍,这表明排放对细颗粒物、可吸入颗粒物和氮氧化物的贡献降低。臭氧与一氧化碳的比值增加了50.1至61.5倍,这意味着二次生成明显增加。封控后,排放对各类污染物的贡献均有所增加。在封控期间,受一些不间断工业生产过程的影响,工业区的细颗粒物浓度下降幅度最小(20.5%)。与封控期间相比,封控解除后居民活动、交通和工业生产基本恢复,导致与细颗粒物排放相关的浓度下降幅度有所缓解。与排放相关的臭氧浓度增加可能与封控期间氮氧化物和细颗粒物浓度下降有关。臭氧浓度升高部分抵消了氮氧化物和细颗粒物浓度降低带来的空气质量改善。封控解除后,郊区和城市背景站点与气象相关的臭氧浓度分别增加了16.2微克·立方米和16.1微克·立方米,这可能归因于环境温度升高和相对湿度降低。三环线交通区和中心城区因交通和工业排放减少导致的细颗粒物浓度下降和臭氧浓度增加,可为当前子区域内细颗粒物和臭氧的协同精准管控提供参考。

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