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基于连续统中的小型化束缚态,通过氮化硅光子晶体腔增强CdSe/ZnS量子点的自发发射。

Enhancement of spontaneous emission from CdSe/ZnS quantum dots through silicon nitride photonic crystal cavity based on miniaturized bound states in the continuum.

作者信息

Qiu Guixin, Wei Dunzhao, Liu Zhuojun, Liu Jin

机构信息

State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics, Sun Yat-sen University, Guangzhou 510275, China.

State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, Beijing 100871, China.

出版信息

Nanoscale. 2023 Feb 23;15(8):3757-3763. doi: 10.1039/d2nr05031e.

Abstract

Colloidal CdSe/ZnS quantum dots (QDs) exhibit excellent optical properties for wide potential applications in light-emitting diodes, solar concentrators, and single-photon sources. However, the ultra-thin films with low concentration of QDs still encounter inefficient photoluminescence (PL) and poor directionality of radiation, which need to be enhanced using nanophotonics device designs. Here we design and experimentally demonstrate an on-substrate silicon nitride (SiN) photonic crystal (PhC) microcavity encapsulated by a layer of PMMA hosting CdSe/ZnS QDs. The miniaturized bound states in the continuum (BIC) supported by our structures, provide high- resonant modes with highly-directional emission patterns. Experimental results show that the BIC mode in the microcavity has a -factor up to 7000 owing to the symmetric refractive index distribution along the -direction, rendering 8.5-fold enhancement of PL intensity and 8.4-fold acceleration of radiative emission rate. Our work provides a practical way for constructing efficient on-chip surface-emitting light sources on silicon-based integrated photonic devices.

摘要

胶体CdSe/ZnS量子点(QDs)具有优异的光学性能,在发光二极管、太阳能聚光器和单光子源等广泛的潜在应用中表现出色。然而,具有低浓度量子点的超薄膜仍然存在光致发光(PL)效率低下和辐射方向性差的问题,需要通过纳米光子器件设计来增强。在此,我们设计并通过实验证明了一种在衬底上的氮化硅(SiN)光子晶体(PhC)微腔,该微腔由一层含有CdSe/ZnS量子点的聚甲基丙烯酸甲酯(PMMA)封装。我们的结构所支持的连续体中的束缚态(BIC)的小型化,提供了具有高方向性发射模式的高谐振模式。实验结果表明,由于沿z方向的对称折射率分布,微腔中的BIC模式具有高达7000的品质因数,使PL强度提高了8.5倍,辐射发射速率加快了8.4倍。我们的工作为在硅基集成光子器件上构建高效的片上表面发射光源提供了一条实用途径。

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