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Mg/MgH的储氢性能及其改进措施：研究进展与趋势

Hydrogen Storage Performance of Mg/MgH and Its Improvement Measures: Research Progress and Trends.

作者信息

Yang Xinglin, Li Wenxuan, Zhang Jiaqi, Hou Quanhui

机构信息

School of Energy and Power, Jiangsu University of Science and Technology, Zhenjiang 212003, China.

School of Automotive Engineering, Yancheng Institute of Technology, Yancheng 224051, China.

出版信息

Materials (Basel). 2023 Feb 14;16(4):1587. doi: 10.3390/ma16041587.

DOI:10.3390/ma16041587
PMID:36837217
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9966284/
Abstract

Due to its high hydrogen storage efficiency and safety, Mg/MgH stands out from many solid hydrogen storage materials and is considered as one of the most promising solid hydrogen storage materials. However, thermodynamic/kinetic deficiencies of the performance of Mg/MgH limit its practical applications for which a series of improvements have been carried out by scholars. This paper summarizes, analyzes and organizes the current research status of the hydrogen storage performance of Mg/MgH and its improvement measures, discusses in detail the hot studies on improving the hydrogen storage performance of Mg/MgH (improvement measures, such as alloying treatment, nano-treatment and catalyst doping), and focuses on the discussion and in-depth analysis of the catalytic effects and mechanisms of various metal-based catalysts on the kinetic and cyclic performance of Mg/MgH. Finally, the challenges and opportunities faced by Mg/MgH are discussed, and strategies to improve its hydrogen storage performance are proposed to provide ideas and help for the next research in Mg/MgH and the whole field of hydrogen storage.

摘要

由于其高储氢效率和安全性，Mg/MgH在众多固体储氢材料中脱颖而出，被认为是最具潜力的固体储氢材料之一。然而，Mg/MgH性能的热力学/动力学缺陷限制了其实际应用，学者们为此进行了一系列改进。本文总结、分析并整理了Mg/MgH储氢性能及其改进措施的当前研究现状，详细讨论了改善Mg/MgH储氢性能的热点研究（改进措施，如合金化处理、纳米处理和催化剂掺杂），重点讨论并深入分析了各种金属基催化剂对Mg/MgH动力学和循环性能的催化作用及机理。最后，讨论了Mg/MgH面临的挑战与机遇，并提出了提高其储氢性能的策略，为Mg/MgH及整个储氢领域的后续研究提供思路和帮助。

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NiFe/BC nanocatalysts based on biomass charcoal self-reduction achieves excellent hydrogen storage performance of MgH.基于生物质炭自还原的镍铁/生物质炭纳米催化剂实现了氢化镁优异的储氢性能。
Dalton Trans. 2022 Oct 11;51(39):14960-14969. doi: 10.1039/d2dt02425j.
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Oxygen Vacancy-Rich 2D TiO Nanosheets: A Bridge Toward High Stability and Rapid Hydrogen Storage Kinetics of Nano-Confined MgH.
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Nanomicro Lett. 2022 Jul 15;14(1):144. doi: 10.1007/s40820-022-00891-9.
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5
Nanostructural Perspective for Destabilization of Mg Hydride Using the Immiscible Transition Metal Mn.利用不混溶过渡金属锰使氢化镁失稳的纳米结构视角
Inorg Chem. 2021 Oct 4;60(19):15024-15030. doi: 10.1021/acs.inorgchem.1c02525. Epub 2021 Sep 20.
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