• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利：CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法，用中文像聊天一样搜索，搜遍4000万医学文献。AI智能推荐，让科研检索更轻松。

立即免费搜索

文件翻译

保留排版，准确专业，支持PDF/Word/PPT等文件格式，支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述，25分钟生成高质量综述，智能提取关键信息，辅助科研写作。

立即免费体验

采用水热法制备的可回收 MXene 修饰的 BiFeO3 纳米复合材料有效去除磺胺类药物。

Effective Removal of Sulfonamides Using Recyclable MXene-Decorated Bismuth Ferrite Nanocomposites Prepared via Hydrothermal Method.

机构信息

CAS Key Laboratory of Chemistry of Northwestern Plant Resources and Key Laboratory for Natural Medicine of Gansu Province, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China.

University of Chinese Academy of Sciences, Beijing 100049, China.

出版信息

Molecules. 2023 Feb 5;28(4):1541. doi: 10.3390/molecules28041541.

DOI:10.3390/molecules28041541
PMID:36838529
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9962683/
Abstract

Developing a simple and efficient method for removing organic micropollutants from aqueous systems is crucial. The present study describes the preparation and application, for the first time, of novel MXene-decorated bismuth ferrite nanocomposites (BiFeO/MXene) for the removal of six sulfonamides including sulfadiazine (SDZ), sulfathiazole (STZ), sulfamerazine (SMZ), sulfamethazine (SMTZ), sulfamethoxazole (SMXZ) and sulfisoxazole (SXZ). The properties of BiFeO/MXene are enhanced by the presence of BiFeO nanoparticles, which provide a large surface area to facilitate the removal of sulfonamides. More importantly, BiFeO/MXene composites demonstrated remarkable sulfonamide adsorption capabilities compared to pristine MXene, which is due to the synergistic effect between BiFeO and MXene. The kinetics and isotherm models of sulfonamide adsorption on BiFeO/MXene are consistent with a pseudo-second-order kinetics and Langmuir model. BiFeO/MXene had appreciable reusability after five adsorption-desorption cycles. Furthermore, BiFeO/MXene is stable and retains its original properties upon desorption. The present work provides an effective method for eliminating sulfonamides from water by exploiting the excellent texture properties of BiFeO/MXene.

摘要

开发一种简单高效的方法从水相中去除有机微量污染物至关重要。本研究首次描述了新型 MXene 修饰的铋铁氧体纳米复合材料 (BiFeO/MXene) 的制备和应用，用于去除包括磺胺嘧啶 (SDZ)、磺胺噻唑 (STZ)、磺胺甲嘧啶 (SMZ)、磺胺二甲嘧啶 (SMTZ)、磺胺甲噁唑 (SMXZ) 和磺胺异噁唑 (SXZ) 在内的六种磺胺类抗生素。BiFeO 纳米粒子的存在增强了 BiFeO/MXene 的性能，提供了更大的表面积，有利于磺胺类抗生素的去除。更重要的是，与原始 MXene 相比，BiFeO/MXene 复合材料表现出显著的磺胺类抗生素吸附能力，这是由于 BiFeO 和 MXene 之间的协同效应。磺胺类抗生素在 BiFeO/MXene 上的吸附动力学和等温线模型符合准二级动力学和 Langmuir 模型。BiFeO/MXene 在经过五次吸附-解吸循环后具有相当的可重复使用性。此外，BiFeO/MXene 在解吸后稳定且保留其原始特性。本工作提供了一种通过利用 BiFeO/MXene 的优异质地特性从水中去除磺胺类抗生素的有效方法。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/2935a8323a4c/molecules-28-01541-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/0a6c6341489e/molecules-28-01541-sch001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/e5d4536d2d53/molecules-28-01541-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/e94ba2b1e9f8/molecules-28-01541-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/33b7fdc7883c/molecules-28-01541-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/666c8561939b/molecules-28-01541-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/c4ebdd8f557c/molecules-28-01541-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/2935a8323a4c/molecules-28-01541-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/0a6c6341489e/molecules-28-01541-sch001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/e5d4536d2d53/molecules-28-01541-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/e94ba2b1e9f8/molecules-28-01541-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/33b7fdc7883c/molecules-28-01541-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/666c8561939b/molecules-28-01541-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/c4ebdd8f557c/molecules-28-01541-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7bf7/9962683/2935a8323a4c/molecules-28-01541-g006.jpg

相似文献

1
Effective Removal of Sulfonamides Using Recyclable MXene-Decorated Bismuth Ferrite Nanocomposites Prepared via Hydrothermal Method.采用水热法制备的可回收 MXene 修饰的 BiFeO3 纳米复合材料有效去除磺胺类药物。
Molecules. 2023 Feb 5;28(4):1541. doi: 10.3390/molecules28041541.
2
Synthesis and application of bismuth ferrite nanosheets supported functionalized carbon nanofiber for enhanced electrochemical detection of toxic organic compound in water samples.基于功能化碳纤维负载的铁酸铋纳米片的合成及其在水样中有毒有机化合物电化学检测中的应用。
J Colloid Interface Sci. 2018 Mar 15;514:59-69. doi: 10.1016/j.jcis.2017.12.016. Epub 2017 Dec 6.
3
Preparation of Fe/Ni Bimetallic Oxide Porous Graphene Composite Materials for Efficient Adsorption and Removal of Sulfonamides.用于高效吸附和去除磺胺类药物的 Fe/Ni 双金属氧化物多孔石墨烯复合材料的制备。
Langmuir. 2021 Oct 19;37(41):12242-12253. doi: 10.1021/acs.langmuir.1c02275. Epub 2021 Oct 8.
4
Novel magnetic nanocomposites BiFeO/Cu(BDC) for efficient dye removal.用于高效去除染料的新型磁性纳米复合材料BiFeO/Cu(BDC)
Heliyon. 2023 Oct 21;9(11):e20689. doi: 10.1016/j.heliyon.2023.e20689. eCollection 2023 Nov.
5
BiFeO immobilized within liquid natural rubber-based hydrogel with enhanced adsorption-photocatalytic performance.BiFeO 固载于液体天然橡胶基水凝胶中，具有增强的吸附-光催化性能。
Int J Biol Macromol. 2021 Jul 1;182:1495-1506. doi: 10.1016/j.ijbiomac.2021.05.104. Epub 2021 May 18.
6
Linearized and nonlinearized modellings for comparative uptake assessment of metal-organic framework-derived nanocomposite towards sulfonamide antibiotics.线性化和非线性化建模用于比较金属有机骨架衍生纳米复合材料对磺胺类抗生素的摄取评估。
Environ Sci Pollut Res Int. 2021 Dec;28(45):63448-63463. doi: 10.1007/s11356-020-09312-z. Epub 2020 Jun 25.
7
Preparation of β-cyclodextrin/dopamine hydrochloride-graphene oxide and its adsorption properties for sulfonamide antibiotics.β-环糊精/盐酸多巴胺-氧化石墨烯的制备及其对磺胺类抗生素的吸附性能。
Environ Sci Pollut Res Int. 2022 Oct;29(46):70192-70201. doi: 10.1007/s11356-022-20828-4. Epub 2022 May 18.
8
Enhanced adsorption performance and regeneration of magnetic FeO nanoparticles assisted extracellular polymeric substances in sulfonamide-contaminated water.磁性 FeO 纳米颗粒增强吸附性能及在外源性聚合物辅助下对磺胺类污染物污染水体的再生。
Environ Sci Pollut Res Int. 2020 Feb;27(5):4866-4875. doi: 10.1007/s11356-019-06956-4. Epub 2019 Dec 16.
9
Facile synthesis of magnetic CoO/BFO nanocomposite for effective reduction of nitrophenol isomers.用于有效还原硝基酚异构体的磁性 CoO/BFO 纳米复合材料的简便合成。
Chemosphere. 2019 Mar;219:914-922. doi: 10.1016/j.chemosphere.2018.12.045. Epub 2018 Dec 6.
10
Design and Preparation of Chitosan-Crosslinked Bismuth Ferrite/Biochar Coupled Magnetic Material for Methylene Blue Removal.壳聚糖交联的四氧化三铁/生物炭复合磁性材料的设计与制备及其对亚甲基蓝的去除。
Int J Environ Res Public Health. 2019 Dec 18;17(1):6. doi: 10.3390/ijerph17010006.

本文引用的文献

1
Advances in BiWO-Based Photocatalysts for Degradation of Organic Pollutants.基于 BiWO 的光催化剂在有机污染物降解方面的研究进展。
Molecules. 2022 Dec 8;27(24):8698. doi: 10.3390/molecules27248698.
2
One-Pot Synthesis of Cellulose/MXene/PVA Foam for Efficient Methylene Blue Removal.一锅法合成纤维素/MXene/PVA 泡沫用于高效去除亚甲基蓝。
Molecules. 2022 Jun 30;27(13):4243. doi: 10.3390/molecules27134243.
3
Two-Dimensional Imprinting Strategy to Create Specific Nanotrap for Selective Uranium Adsorption with Ultrahigh Capacity.
用于创建具有超高容量的选择性铀吸附特定纳米陷阱的二维印迹策略
ACS Appl Mater Interfaces. 2022 Feb 23;14(7):9408-9417. doi: 10.1021/acsami.1c20543. Epub 2022 Feb 11.
4
Adsorption behaviors and mechanisms of Fe/Mg layered double hydroxide loaded on bentonite on Cd (II) and Pb (II) removal.负载于膨润土上的 Fe/Mg 层状双氢氧化物对 Cd(II)和 Pb(II)去除的吸附行为和机制。
J Colloid Interface Sci. 2022 Apr 15;612:572-583. doi: 10.1016/j.jcis.2021.12.151. Epub 2021 Dec 28.
5
Adsorption behavior and mechanism of sulfonamides on controllably synthesized covalent organic frameworks.磺胺类药物在可控合成共价有机骨架上的吸附行为和机理。
Environ Sci Pollut Res Int. 2022 Mar;29(13):18680-18688. doi: 10.1007/s11356-021-17169-z. Epub 2021 Oct 25.
6
Preparation of Fe/Ni Bimetallic Oxide Porous Graphene Composite Materials for Efficient Adsorption and Removal of Sulfonamides.用于高效吸附和去除磺胺类药物的 Fe/Ni 双金属氧化物多孔石墨烯复合材料的制备。
Langmuir. 2021 Oct 19;37(41):12242-12253. doi: 10.1021/acs.langmuir.1c02275. Epub 2021 Oct 8.
7
Iron oxide (FeO)-laden titanium carbide (TiCT) MXene stacks for the efficient sequestration of cationic dyes from aqueous solution.负载氧化铁（FeO）的碳化钛（TiCT）MXene 层用于从水溶液中高效捕获阳离子染料。
Chemosphere. 2022 Jan;286(Pt 2):131679. doi: 10.1016/j.chemosphere.2021.131679. Epub 2021 Aug 3.
8
Removal of ibuprofen from aqueous media by adsorption: A comprehensive review.吸附法去除水相中的布洛芬：综述。
Sci Total Environ. 2021 Aug 1;780:146608. doi: 10.1016/j.scitotenv.2021.146608. Epub 2021 Mar 19.
9
TiCTMXene/nitrogen-doped reduced graphene oxide composite: a high-performance electrochemical sensing platform for adrenaline detection.TiCTMXene/氮掺杂还原氧化石墨烯复合材料：用于检测肾上腺素的高性能电化学传感平台。
Nanotechnology. 2021 Apr 6;32(26). doi: 10.1088/1361-6528/abef94.
10
Coating magnetite alters the mechanisms and site energy for sulfonamide antibiotic sorption on biochar.涂层磁铁矿改变了磺胺类抗生素在生物炭上吸附的机制和位置能。
J Hazard Mater. 2021 May 5;409:125024. doi: 10.1016/j.jhazmat.2020.125024. Epub 2021 Jan 2.