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人为活动控制内陆河下游沉积物有机碳的源动态。

Anthropogenic activities control the source dynamics of sediment organic carbon in the lower reach of an inland river.

机构信息

School of Geographical Sciences, Hunan Normal University, Changsha 410081, China.

School of Geographical Sciences, Hunan Normal University, Changsha 410081, China; College of Environmental Science and Engineering, Hunan University, Changsha 410082, China.

出版信息

Water Res. 2023 Apr 15;233:119779. doi: 10.1016/j.watres.2023.119779. Epub 2023 Feb 22.

Abstract

Sediment organic carbon (SeOC) sources with rich information can be used as a "historical archive" reflecting anthropogenic activities in the catchment, which is crucial to carbon management in the watershed. Anthropogenic activities and hydrodynamic conditions significantly influence the river environment and are reflected by the SeOC sources. However, the key drivers of the SeOC source dynamics are ambiguous, which restricts the behavior of regulating the carbon output of the basin. In this study, sediment cores from the lower reach of an inland river were selected to quantify the SeOC sources based on a centennial scale. A partial least squares path model was used to establish the relationship between anthropogenic activities and hydrological conditions with the SeOC sources. Findings showed that the exogenous advantage of SeOC composition was gradually significant (early period: 54.3%; middle period: 81%; later period: 82%) from the bottom layer to the surface layer of the sediments in the lower reach of the Xiangjiang River. Factors related to anthropogenic activities controlled the external input of SeOC (δC: r = -0.94, P < 0.001; δN: r = -0.66, P < 0.001). Different anthropogenic activities performed different effects. Land use change aggravated soil erosion and brought more terrestrial organic carbon to the downstream. The variation of grassland carbon input was the most obvious (from 33.6% to 18.4%). In contrast, the reservoir construction intercepted upstream sediments, which might have been the main reason for the slow growth of terrestrial organic carbon input in the downstream in the later period. This study provides a specific grafting for the SeOC records - source changes - anthropogenic activities in the lower reach of the river, which provides scientific basis for watershed carbon management.

摘要

河流沉积物中的有机碳(SeOC)来源可以作为反映流域人为活动的“历史档案”,这对于流域的碳管理至关重要。人为活动和水动力条件显著影响河流环境,并且可以通过 SeOC 来源来反映。然而,SeOC 源动力的关键驱动因素尚不清楚,这限制了对流域碳输出进行调节的行为。在这项研究中,选择内陆河流下游的沉积物岩芯,基于百年尺度量化了 SeOC 来源。采用偏最小二乘路径模型建立了人为活动和水文条件与 SeOC 来源之间的关系。研究结果表明,湘江下游沉积物表层到底层,外源优势的 SeOC 组成逐渐显著(早期:54.3%;中期:81%;后期:82%)。与人为活动相关的因素控制着 SeOC 的外部输入(δC:r = -0.94,P < 0.001;δN:r = -0.66,P < 0.001)。不同的人为活动产生了不同的影响。土地利用变化加剧了土壤侵蚀,将更多的陆地有机碳带入下游。草地碳输入的变化最为明显(从 33.6%降至 18.4%)。相比之下,水库建设拦截了上游沉积物,这可能是下游陆地有机碳输入在后期增长缓慢的主要原因。本研究为河流下游的 SeOC 记录-源变化-人为活动提供了具体的研究结果,为流域碳管理提供了科学依据。

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