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农业土壤风蚀对 WRF-Chem 和 WEPS 模拟的城市 PM 浓度的影响:以中国开封为例。

Effect of agricultural soil wind erosion on urban PM concentrations simulated by WRF-Chem and WEPS: A case study in Kaifeng, China.

机构信息

Laboratory of Geospatial Technology for the Middle and Lower Yellow River Regions, Ministry of Education, Henan University, Kaifeng, Henan, 475004, China; Institute of Urban Big Data, College of Geography and Environmental Science, Henan University, Kaifeng, Henan, 475004, China.

Laboratory of Geospatial Technology for the Middle and Lower Yellow River Regions, Ministry of Education, Henan University, Kaifeng, Henan, 475004, China; Henan Key Laboratory of Integrated Air Pollution Control and Ecological Security, Henan University, Kaifeng, Henan, 475004, China.

出版信息

Chemosphere. 2023 May;323:138250. doi: 10.1016/j.chemosphere.2023.138250. Epub 2023 Feb 25.

Abstract

Dust emission induced by agricultural soil wind erosion is one of the main sources of atmospheric particulate matter (PM) in dryland areas. However, most current air quality models do not consider this emission source, resulting in large uncertainties in PM simulations. Here we estimated the agricultural PM (particulate matter with an aerodynamic diameter <2.5 μm) emission around Kaifeng, a prefecture-level city in central China, using the Wind Erosion Prediction System (WEPS), with the MEIC (Multi-resolution Emission Inventory for China) as an anthropogenic emission source. We then plugged these estimates into the Weather Research and Forecasting model coupled with chemistry (WRF-Chem) to simulate an air pollution episode in Kaifeng, China. Results showed that the addition of agricultural soil PM emissions significantly improved the ability of WRF-Chem to accurately simulate PM concentrations. The PM concentration mean bias and correlation coefficient of not considered and considered agricultural dust emission were -72.35 μg m and 3.31 μg m and 0.3 and 0.58, respectively. The PM emitted by the agricultural soil wind erosion contributed around 37.79% of the PM in the Kaifeng municipal district during this pollution episode. This study confirmed that the dust emission caused by agricultural soil wind erosion can significantly impact urban PM concentrations which surrounded by large areas of farmland, and also indicated that coupling dust emissions from farmland with anthropogenic air pollutant emissions can improve the accuracy of air quality models.

摘要

农业土壤风蚀引起的扬尘是旱地地区大气颗粒物(PM)的主要来源之一。然而,大多数当前的空气质量模型并未考虑这一排放源,导致 PM 模拟存在较大不确定性。本研究使用风蚀预测系统(WEPS),并结合中国多分辨率排放清单(MEIC)作为人为排放源,对中国中部地级市开封周围的农业 PM(空气动力学直径<2.5 μm 的颗粒物)排放进行了估算。然后,我们将这些估算值输入到天气研究和预报模型耦合化学(WRF-Chem)中,以模拟中国开封的一次空气污染事件。结果表明,添加农业土壤 PM 排放后,WRF-Chem 能够更准确地模拟 PM 浓度。未考虑和考虑农业扬尘排放的 PM 浓度平均偏差和相关系数分别为-72.35μg/m 和 3.31μg/m,以及 0.3 和 0.58。在这次污染事件中,农业土壤风蚀产生的 PM 约占开封市区 PM 的 37.79%。本研究证实,农业土壤风蚀引起的扬尘排放可显著影响周边大面积农田的城市 PM 浓度,也表明将农田扬尘排放与人为空气污染物排放相耦合可以提高空气质量模型的准确性。

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