School of Energy and Power Engineering, Jiangsu University, Zhenjiang 212013, China.
School of Energy and Power Engineering, Jiangsu University, Zhenjiang 212013, China.
J Hazard Mater. 2023 Jun 5;451:131100. doi: 10.1016/j.jhazmat.2023.131100. Epub 2023 Feb 27.
Plasma-catalysis has been recognized as a promising method to decompose hazardous volatile organic compounds (VOCs) since many years ago. To understand the fundamental mechanisms of VOCs decomposition by plasma-catalysis systems, both experimental and modeling studies have been extensively carried out. However, literature on summarized modeling methodologies is still scarce. In this short review, we therefore present a comprehensive overview of modeling methodologies ranging from microscopic to macroscopic modeling in plasma-catalysis for VOCs decomposition. The modeling methods of VOCs decomposition by plasma and plasma-catalysis are classified and summarized. The roles of plasma and plasma-catalyst interactions in VOCs decomposition are also critically examined. Taking the current advances in understanding the decomposition mechanisms of VOCs into account, we finally provide our perspectives for future research directions. This short review aims to stimulate the further development of plasma-catalysis for VOCs decomposition in both fundamental studies and practical applications with advanced modeling methods.
多年以来,等离子体催化已被认为是一种很有前途的方法,可以分解危险的挥发性有机化合物(VOCs)。为了理解等离子体催化体系分解 VOCs 的基本机制,已经广泛开展了实验和建模研究。然而,关于总结建模方法的文献仍然很少。因此,在这篇简短的综述中,我们全面概述了从微观到宏观的等离子体催化 VOCs 分解的建模方法。对等离子体和等离子体催化分解 VOCs 的建模方法进行了分类和总结。还批判性地检验了等离子体和等离子体催化剂相互作用在 VOCs 分解中的作用。考虑到目前对 VOCs 分解机制的理解进展,我们最后为未来的研究方向提供了我们的看法。这篇简短的综述旨在通过先进的建模方法,激发在基础研究和实际应用中进一步发展等离子体催化分解 VOCs。