Graduate School of Engineering, Nagoya University, Nagoya, 464-8603, Japan.
CREST, Japan Science and Technology Agency, Kawaguchi, 332-0012, Japan.
Sci Rep. 2023 Mar 17;13(1):4425. doi: 10.1038/s41598-023-31420-2.
We report on the observation of sign reversal of vortex-Nernst effect in epitaxial NbN/Fe bilayers deposited on MgO (001) substrates. Strong coupling between vortex magnetisation and ferromagnetic magnetisation at the NbN/Fe bilayer interface is presented. In NbN/Fe bilayer thin films an apparent sign reversal of vortex-Nernst signal under a temperature gradient with magnetic field and temperature is observed when the thickness of Fe is increased up to 5 nm. This reversal of the vortex-Nernst effect is associated with the enhancement of the spin Seebeck effects (SSE) near T due to coherence peak effect (CPE) and strong coupling of vortex magnetisation and ferromagnetic magnetisation at the interface of the NbN/Fe bilayer. The observed large SSE via inverse spin Hall effect (ISHE) is due to the CPE below and close to T, highlighting the high spin to charge conversion efficiency of NbN in this region. This work may contribute to the development of superconducting spintronic devices by engineering the coupling of the superconductor/ferromagnet interface.
我们报告了在 MgO(001) 衬底上外延生长的 NbN/Fe 双层膜中观察到的涡旋诺尔斯特效应的符号反转。在 NbN/Fe 双层薄膜中,当 Fe 的厚度增加到 5nm 时,在磁场和温度梯度下观察到涡旋诺尔斯特信号的明显符号反转。这种涡旋诺尔斯特效应的反转与由于相干峰效应(CPE)和 NbN/Fe 双层界面处涡旋磁化和铁磁磁化的强耦合导致的 T 附近自旋塞贝克效应(SSE)的增强有关。通过反自旋霍尔效应(ISHE)观察到的大 SSE 是由于 CPE 低于 T 且接近 T,突出了 NbN 在该区域的高自旋到电荷转换效率。这项工作通过工程设计超导体/铁磁体界面的耦合,可能有助于超导自旋电子器件的发展。