Canale Vittorio, Czekajewska Joanna, Klesiewicz Karolina, Papież Monika, Kuziak Agata, Witek Karolina, Piska Kamil, Niemiec Dagmara, Kasza Patryk, Pękala Elżbieta, Empel Joanna, Tomczak Magdalena, Karczewska Elżbieta, Zajdel Paweł
Faculty of Pharmacy, Jagiellonian University Medical College, 9 Medyczna Street, 30-688, Krakow, Poland.
Faculty of Pharmacy, Jagiellonian University Medical College, 9 Medyczna Street, 30-688, Krakow, Poland.
Eur J Med Chem. 2023 May 5;251:115224. doi: 10.1016/j.ejmech.2023.115224. Epub 2023 Mar 6.
The alarming increase in the resistance of bacteria to the currently available antibiotics necessitates the development of new effective antimicrobial agents that are active against bacterial pathogens causing major public health problems. For this purpose, our in-house libraries were screened against a wide panel of clinically relevant Gram-positive and Gram-negative bacteria, based on which compound I was selected for further optimization. Synthetic efforts in a group of arylurea derivatives of aryloxy(1-phenylpropyl) alicyclic diamines, followed with an in vitro evaluation of the activity against multidrug-resistant strains identified compound 44 (1-(3-chlorophenyl)-3-(1-{3-phenyl-3-[3-(trifluoromethyl)phenoxy] propyl}piperidin-4-yl)urea). Compound 44 showed antibacterial activity against Gram-positive bacteria including fatal drug-resistant strains i.e., Staphylococcus aureus (methicillin-resistant, MRSA; vancomycin-intermediate, VISA) and Enterococcus faecium (vancomycin-resistant, VREfm) at low concentrations (0.78-3.125 μg/mL) comparable to last resort antibiotics (i.e., vancomycin and linezolid). It is also potent against biofilm-forming S. aureus and Staphylococcus epidermidis (including linezolid-resistant, LRSE) strains, but with no activity against Gram-negative bacteria (Escherichia coli, Klebsiella pneumoniae and Pseudomonas aeruginosa). Compound 44 showed strong bactericidal properties against susceptible and drug-resistant Gram-positive bacteria. Depolarization of the bacterial cytoplasmic membrane induced by compound 44 suggests a dissipation of the bacterial membrane potential as its mechanism of antibacterial action. The high antimicrobial activity of compound 44, along with its selectivity over mammalian cells (lung MCR-5 and skin BJ fibroblast cell lines) and no hemolytic properties toward horse erythrocytes, proposes arylurea derivatives of aryloxy(1-phenylpropyl) alicyclic diamines for development of novel antibacterial agents.
细菌对现有抗生素的耐药性惊人增加,因此有必要开发对引起重大公共卫生问题的细菌病原体具有活性的新型有效抗菌剂。为此,我们利用内部文库针对一系列临床相关的革兰氏阳性和革兰氏阴性细菌进行筛选,在此基础上选择了化合物I进行进一步优化。对一组芳氧基(1-苯基丙基)脂环族二胺的芳基脲衍生物进行了合成研究,随后对其抗多药耐药菌株的活性进行了体外评估,确定了化合物44(1-(3-氯苯基)-3-(1-{3-苯基-3-[3-(三氟甲基)苯氧基]丙基}哌啶-4-基)脲)。化合物44在低浓度(0.78 - 3.125μg/mL)下对革兰氏阳性菌具有抗菌活性,包括致命的耐药菌株,即金黄色葡萄球菌(耐甲氧西林,MRSA;万古霉素中介,VISA)和粪肠球菌(耐万古霉素,VREfm),其活性与最后手段抗生素(即万古霉素和利奈唑胺)相当。它对形成生物膜的金黄色葡萄球菌和表皮葡萄球菌(包括耐利奈唑胺,LRSE)菌株也有效,但对革兰氏阴性菌(大肠杆菌、肺炎克雷伯菌和铜绿假单胞菌)无活性。化合物44对敏感和耐药革兰氏阳性菌均表现出强大的杀菌特性。化合物44诱导细菌细胞质膜去极化,表明细菌膜电位的消散是其抗菌作用机制。化合物44的高抗菌活性,以及其对哺乳动物细胞(肺MCR-5和皮肤BJ成纤维细胞系)的选择性和对马红细胞无溶血特性,表明芳氧基(1-苯基丙基)脂环族二胺的芳基脲衍生物可用于开发新型抗菌剂。