Saleem Yasser, Sadecka Katarzyna, Korkusinski Marek, Miravet Daniel, Dusko Amintor, Hawrylak Pawel
Department of Physics, University of Ottawa, Ottawa K1N6N5, Canada.
Institute of Theoretical Physics, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, 50-370 Wrocław, Poland.
Nano Lett. 2023 Apr 12;23(7):2998-3004. doi: 10.1021/acs.nanolett.3c00406. Epub 2023 Mar 24.
We present a theory of excitons in gated bilayer graphene (BLG) quantum dots (QDs). Electrical gating of BLG opens an energy gap, turning this material into an electrically tunable semiconductor. Unlike in laterally gated semiconductor QDs, where electrons are attracted and holes repelled, we show here that lateral structuring of metallic gates results in a gated lateral QD confining both electrons and holes. Using an accurate atomistic approach and exact diagonalization tools, we describe strongly interacting electrons and holes forming an electrically tunable exciton. We find these excitons to be different from those found in semiconductor QDs and nanocrystals, with exciton energy tunable by voltage from the terahertz to far infrared (FIR) range. The conservation of spin, valley, and orbital angular momentum results in an exciton fine structure with a band of dark low-energy states, making this system a promising candidate for storage, detection and emission of photons in the terahertz range.
我们提出了一种关于门控双层石墨烯(BLG)量子点(QD)中激子的理论。对BLG进行电门控会打开一个能隙,将这种材料转变为一种电可调谐半导体。与横向门控半导体量子点不同,在横向门控半导体量子点中电子被吸引而空穴被排斥,我们在此表明金属门的横向结构会导致一个门控横向量子点,它能同时限制电子和空穴。使用精确的原子方法和精确对角化工具,我们描述了形成电可调谐激子的强相互作用电子和空穴。我们发现这些激子与半导体量子点和纳米晶体中的激子不同,其激子能量可通过电压在太赫兹到远红外(FIR)范围内进行调谐。自旋、谷和轨道角动量的守恒导致了具有暗低能态能带的激子精细结构,使得该系统成为太赫兹范围内光子存储、检测和发射的有前景的候选者。