Department of Chemistry, University of Oxford, Inorganic Chemistry Laboratory, South Parks Road, Oxford OX1 3QR, UK.
Department of Chemistry, University of Oxford, Inorganic Chemistry Laboratory, South Parks Road, Oxford OX1 3QR, UK.
Bioorg Med Chem. 2023 Apr 1;83:117255. doi: 10.1016/j.bmc.2023.117255. Epub 2023 Mar 21.
Barriers to the ready adoption of biocatalysis into asymmetric synthesis for early stage medicinal chemistry are addressed, using ketone reduction by alcohol dehydrogenase as a model reaction. An efficient substrate screening approach is used to show the wide substrate scope of commercial alcohol dehydrogenase enzymes, with a high tolerance to chemical groups employed in drug discovery (heterocycle, trifluoromethyl and nitrile/nitro groups) observed. We use our screening data to build a preliminary predictive pharmacophore-based screening tool using Forge software, with a precision of 0.67/1, demonstrating the potential for developing substrate screening tools for commercially available enzymes without publicly available structures. We hope that this work will facilitate a culture shift towards adopting biocatalysis alongside traditional chemical catalytic methods in early stage drug discovery.
针对在早期药物化学中引入生物催化进行不对称合成所面临的障碍,我们以醇脱氢酶催化酮还原反应为例进行了探讨。采用一种高效的底物筛选方法,展示了商业醇脱氢酶的广泛底物范围,对药物发现中常用的化学基团(杂环、三氟甲基和腈/硝基)具有较高的耐受性。我们利用筛选数据,使用 Forge 软件构建了一个初步的基于药效团的预测性筛选工具,其精确性为 0.67/1,这表明有可能为商业上可获得的酶开发无需公开结构的底物筛选工具。我们希望这项工作将有助于在早期药物发现中培养一种将生物催化与传统化学催化方法相结合的文化转变。