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用于超小腔光通量映射的被动原子级光学传感器。

Passive atomic-scale optical sensors for mapping light flux in ultra-small cavities.

机构信息

Department of Physics, Technical University of Denmark, DTU Risø Campus, 4000, Roskilde, Denmark.

Department of Geography & Earth Sciences, University of North Carolina at Charlotte, Charlotte, NC, USA.

出版信息

Sci Rep. 2023 Mar 31;13(1):5309. doi: 10.1038/s41598-023-32010-y.

DOI:10.1038/s41598-023-32010-y
PMID:37002276
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10066291/
Abstract

Understanding light propagation and attenuation in cavities is limited by lack of applicable light sensing technologies. Here we demonstrate the use of light-sensitive metastable states in wide bandgap aluminosilicates (feldspar) as passive optical sensors for high-resolution mapping of light flux. We develop non-destructive, infrared photoluminescence (IRPL) imaging of trapped electrons in cracks as thin as 50 µm width to determine the spatio-temporal evolution of light sensitive metastable states in response to light exposure. Modelling of these data yields estimates of relative light flux at different depths along the crack surfaces. Contrary to expectation, the measured light flux does not scale with the crack width, and it is independent of crack orientation suggesting the dominance of diffused light propagation within the cracks. This work paves way for understanding of how light attenuates in the minutest of cavities for applications in areas as diverse as geomorphology, biology/ecology and civil engineering.

摘要

腔内光传播和衰减的理解受到适用光传感技术缺乏的限制。在这里,我们展示了在宽带隙铝硅酸盐(长石)中利用光敏感亚稳态作为被动光学传感器,用于高分辨率通量映射的用途。我们开发了非破坏性的、红外光致发光(IRPL)成像技术,用于探测裂缝中最窄至 50μm 的捕获电子,以确定光敏感亚稳态在光暴露下的时空演化。对这些数据的建模可估算出沿裂缝表面不同深度的相对光通量。与预期相反,测量的光通量与裂缝宽度不成比例,并且与裂缝方向无关,这表明在裂缝内扩散光传播占主导地位。这项工作为理解光在最小的腔体内如何衰减铺平了道路,可应用于地貌学、生物学/生态学和土木工程等各个领域。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/26e0b48f3188/41598_2023_32010_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/d3844d215fc7/41598_2023_32010_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/d43fa8ba969f/41598_2023_32010_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/55a0c4333828/41598_2023_32010_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/caa2d838a4b7/41598_2023_32010_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/770a5a41cd30/41598_2023_32010_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/11b847421ac6/41598_2023_32010_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/26e0b48f3188/41598_2023_32010_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/d3844d215fc7/41598_2023_32010_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/d43fa8ba969f/41598_2023_32010_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/55a0c4333828/41598_2023_32010_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/caa2d838a4b7/41598_2023_32010_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/770a5a41cd30/41598_2023_32010_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/11b847421ac6/41598_2023_32010_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9281/10066291/26e0b48f3188/41598_2023_32010_Fig7_HTML.jpg

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本文引用的文献

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Enhanced Biophotocurrent Generation in Living Photosynthetic Optical Resonator.活体质光合光学谐振器中增强的生物光电流产生
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Optical bleaching front in bedrock revealed by spatially-resolved infrared photoluminescence.通过空间分辨红外光致发光揭示的基岩中的光学漂白前沿。
Sci Rep. 2019 Feb 22;9(1):2611. doi: 10.1038/s41598-019-38815-0.
5
Optical dating in a new light: A direct, non-destructive probe of trapped electrons.光学测年新视角:对捕获电子的直接、无损探测。
Sci Rep. 2017 Sep 26;7(1):12097. doi: 10.1038/s41598-017-10174-8.
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Strong coupling between chlorosomes of photosynthetic bacteria and a confined optical cavity mode.光合细菌中类菌叶绿素与受限光腔模的强耦合。
Nat Commun. 2014 Nov 28;5:5561. doi: 10.1038/ncomms6561.
7
Role of light intensification by cracks in optical breakdown on surfaces.表面光学击穿中裂纹对光增强的作用。
J Opt Soc Am A Opt Image Sci Vis. 2001 Oct;18(10):2607-16. doi: 10.1364/josaa.18.002607.