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平面过渡金属二卤族化合物超晶格中的谷光学吸收。

Valley-optical absorption in planar transition metal dichalcogenide superlattices.

机构信息

Faculty of Physics, University of Tabriz, Tabriz, Iran.

Research Institute for Applied Physics and Astronomy (RIAPA), University of Tabriz, Tabriz, Iran.

出版信息

Sci Rep. 2023 Apr 3;13(1):5439. doi: 10.1038/s41598-023-31950-9.

Abstract

In this study, we investigate the optical absorption of a planar superlattice comprising alternatively arranged two-dimensional Transition Metal DiChalcogenide semiconductors. Within a semi-classical model and using the Dirac-like equation in the presence of light interaction as a perturbation, we obtained the governing Hamiltonian. Using this Hamiltonian, we derived a fully analytical relationship for the absorption coefficient of the structure. By calculating the effective mass for different bands and using the Drude-Lorentz model, our approach is able to determine the oscillator strength and the effective refractive index of the structure. We found that the spin-orbit coupling has important effect on the absorption coefficient and energy bands where it reduces the absorption coefficient of the structure from typical value of [Formula: see text]-[Formula: see text], also the valence band experiences a significant blue shift, while the conduction band shows minor changes due to spin orbit coupling. Moreover, the role of incident light angle and light polarization were studied in details at different valleys of [Formula: see text] and [Formula: see text]. The most important finding is that by changing the polarization of incident light, it is possible to increase the absorption coefficients of [Formula: see text] and [Formula: see text] valleys by up to 30 times. For light propagation direction close to perpendicular to the plane of the superlattice, the right-circular polarization is absorbed only by [Formula: see text] valley in contrast to the left-circular polarization, which is absorbed by the [Formula: see text] valley. Our model might be used to design newly developed 2D optovalleytronic devices.

摘要

在这项研究中,我们研究了由二维过渡金属二硫属化物半导体交替排列构成的平面超晶格的光学吸收。在半经典模型中,我们使用存在光相互作用的狄拉克型方程作为微扰,得到了控制哈密顿量。利用这个哈密顿量,我们推导出了结构吸收系数的全解析关系。通过计算不同能带的有效质量并使用德鲁德-洛伦兹模型,我们的方法能够确定结构的振子强度和有效折射率。我们发现,自旋轨道耦合对吸收系数和能带结构有重要影响,它降低了结构的吸收系数,从典型的[Formula: see text]-[Formula: see text]值,同时价带经历了显著的蓝移,而导带由于自旋轨道耦合只有较小的变化。此外,我们还详细研究了在不同[Formula: see text]和[Formula: see text]谷的入射光角度和光偏振的作用。最重要的发现是,通过改变入射光的偏振,可以将[Formula: see text]和[Formula: see text]谷的吸收系数提高多达 30 倍。对于接近垂直于超晶格平面的光传播方向,右旋圆偏振光仅被[Formula: see text]谷吸收,而左旋圆偏振光则被[Formula: see text]谷吸收。我们的模型可用于设计新开发的二维光谷电子器件。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d538/10070451/059eaa3262f7/41598_2023_31950_Fig1_HTML.jpg

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