Orfila Gloria, Sanchez-Manzano David, Arora Ashima, Cuellar Fabian, Ruiz-Gómez Sandra, Rodriguez-Corvillo Sara, López Sandra, Peralta Andrea, Carreira Santiago J, Gallego Fernando, Tornos Javier, Rouco Victor, Riquelme Juan J, Munuera Carmen, Mompean Federico J, Garcia-Hernandez Mar, Sefrioui Zouhair, Villegas Javier E, Perez Lucas, Rivera-Calzada Alberto, Leon Carlos, Valencia Sergio, Santamaria Jacobo
GFMC, Department Física de Materiales, Facultad de Física, Universidad Complutense, Madrid, 28040, Spain.
Unité Mixte de Physique, CNRS, Thales, Palaiseau, 91767, France.
Adv Mater. 2023 Aug;35(33):e2211176. doi: 10.1002/adma.202211176. Epub 2023 Jul 11.
Generation, manipulation, and sensing of magnetic domain walls are cornerstones in the design of efficient spintronic devices. Half-metals are amenable for this purpose as large low field magnetoresistance signals can be expected from spin accumulation at spin textures. Among half metals, La Sr MnO (LSMO) manganites are considered as promising candidates for their robust half-metallic ground state, Curie temperature above room temperature (T = 360 K, for x = 1/3), and chemical stability. Yet domain wall magnetoresistance is poorly understood, with large discrepancies in the reported values and conflicting interpretation of experimental data due to the entanglement of various source of magnetoresistance, namely, spin accumulation, anisotropic magnetoresistance, and colossal magnetoresistance. In this work, the domain wall magnetoresistance is measured in LSMO cross-shape nanowires with single-domain walls nucleated across the current path. Magnetoresistance values above 10% are found to be originating at the spin accumulation caused by the mistracking effect of the spin texture of the domain wall by the conduction electrons. Fundamentally, this result shows the importance on non-adiabatic processes at spin textures despite the strong Hund coupling to the localized t electrons of the manganite. These large magnetoresistance values are high enough for encoding and reading magnetic bits in future oxide spintronic sensors.
磁畴壁的产生、操控和传感是高效自旋电子器件设计的基石。半金属适用于此目的,因为在自旋纹理处的自旋积累有望产生大的低场磁电阻信号。在半金属中,镧锶锰氧化物(LSMO)因其稳健的半金属基态、高于室温的居里温度(对于x = 1/3,T = 360 K)和化学稳定性而被视为有前景的候选材料。然而,畴壁磁电阻仍未得到很好的理解,由于各种磁电阻来源(即自旋积累、各向异性磁电阻和巨磁电阻)的纠缠,报告值存在很大差异,对实验数据的解释也相互矛盾。在这项工作中,在具有单畴壁且畴壁横跨电流路径成核的LSMO十字形纳米线中测量了畴壁磁电阻。发现超过10%的磁电阻值源于传导电子对畴壁自旋纹理的误跟踪效应所引起的自旋积累。从根本上说,这一结果表明了尽管与锰氧化物的局域t电子存在强洪德耦合,但自旋纹理处的非绝热过程仍很重要。这些大的磁电阻值足以在未来的氧化物自旋电子传感器中对磁位进行编码和读取。