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通过飞秒激光诱导正向转移实现钙钛矿量子点的高分辨率图案化

High-Resolution Patterning of Perovskite Quantum Dots via Femtosecond Laser-Induced Forward Transfer.

作者信息

Liang Shu-Yu, Liu Yue-Feng, Ji Zhi-Kun, Wang Shen-Yuan, Xia Hong, Sun Hong-Bo

机构信息

State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin University, 2699 Qianjin Street, Changchun 130012, People's Republic of China.

State Key Laboratory of Precision Measurement Technology and Instruments, Department of Precision Instrument, Tsinghua University, Beijing 100084, People's Republic of China.

出版信息

Nano Lett. 2023 May 10;23(9):3769-3774. doi: 10.1021/acs.nanolett.3c00006. Epub 2023 Apr 27.

Abstract

High-resolution patterning of perovskite quantum dots (PQDs) is of significant importance for satisfying various practical applications, including high-resolution displays and image sensing. However, due to the limitation of the instability of PQDs, the existing patterning strategy always involves chemical reagent treatment or mask contact that is not suitable for PQDs. Therefore, it is still a challenge to fabricate high-resolution full-color PQD arrays. Here, we present a femtosecond laser-induced forward transfer (FsLIFT) technology, which enables the programmable fabrication of high-resolution full-color PQD arrays and arbitrary micropatterns. The FsLIFT process integrates transfer, deposition, patterning, and alignment in one step without involving a mask and chemical reagent treatment, guaranteeing the preservation of the photophysical properties of PQDs. A full-color PQD array with a high resolution of 2 μm has been successfully achieved. We anticipate that our facile and flexible FsLIFT technology can facilitate the development of diverse practical applications based on patterned PQDs.

摘要

钙钛矿量子点(PQD)的高分辨率图案化对于满足各种实际应用至关重要,包括高分辨率显示器和图像传感。然而,由于PQD稳定性的限制,现有的图案化策略总是涉及化学试剂处理或掩膜接触,这不适用于PQD。因此,制造高分辨率全彩PQD阵列仍然是一个挑战。在此,我们提出了一种飞秒激光诱导正向转移(FsLIFT)技术,该技术能够可编程地制造高分辨率全彩PQD阵列和任意微图案。FsLIFT工艺在一步中集成了转移、沉积、图案化和对准,无需掩膜和化学试剂处理,保证了PQD光物理性质的保留。已经成功实现了分辨率高达2μm的全彩PQD阵列。我们预计,我们简便灵活的FsLIFT技术能够促进基于图案化PQD的各种实际应用的发展。

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