Balan Cristina, van der Jagt Johannes W, Fassatoui Aymen, Peña Garcia Jose, Jeudy Vincent, Thiaville André, Bonfim Marlio, Vogel Jan, Ranno Laurent, Ravelosona Dafiné, Pizzini Stefania
Univ. Grenoble Alpes, CNRS, Institut Néel, Grenoble, 38042, France.
Spin-Ion Technologies, 10 Boulevard Thomas Gobert, Palaiseau, 91120, France.
Small. 2023 Jul;19(29):e2302039. doi: 10.1002/smll.202302039. Epub 2023 May 13.
Ion irradiation with light ions is an appealing way to finely tune the magnetic properties of thin magnetic films and in particular the perpendicular magnetic anisotropy (PMA). In this work, the effect of He irradiation on the magnetization reversal and on the domain wall dynamics of Pt/Co/AlOx trilayers is illustrated. Fluences up to 1.5 × 10 ions cm strongly decrease the PMA, without affecting neither the spontaneous magnetization nor the strength of the interfacial Dzyaloshinskii-Moriya interaction (DMI). This confirms experimentally the robustness of the DMI interaction against interfacial chemical intermixing, already predicted by theory. In parallel with the decrease of the PMA, a strong decrease of the domain wall depinning field is observed after irradiation. This allows the domain walls to reach large maximum velocities with a lower magnetic field compared to that needed for the pristine films. Decoupling PMA from DMI can, therefore, be beneficial for the design of low energy devices based on domain wall dynamics. When the samples are irradiated with larger He fluences, the magnetization gets close to the out-of-plane/in-plane reorientation transition, where ≈100nm size magnetic skyrmions are stabilized. It is observed that as the He fluence increases, the skyrmion size decreases while these magnetic textures become more stable against the application of an external magnetic field, as predicted by theoretical models developed for ultrathin films with labyrinthine domains.
用轻离子进行离子辐照是一种微调磁性薄膜磁性能,特别是垂直磁各向异性(PMA)的有吸引力的方法。在这项工作中,展示了氦离子辐照对Pt/Co/AlOx三层膜的磁化翻转和畴壁动力学的影响。高达1.5×10离子/cm的辐照通量会强烈降低PMA,而不影响自发磁化强度和界面Dzyaloshinskii-Moriya相互作用(DMI)的强度。这通过实验证实了DMI相互作用对界面化学混合的鲁棒性,这一点理论上早已预测到。与PMA的降低同时,辐照后观察到畴壁脱钉场大幅降低。这使得畴壁在比原始薄膜所需磁场更低的磁场下就能达到较大的最大速度。因此,将PMA与DMI解耦对于基于畴壁动力学的低能耗器件设计可能是有益的。当样品用更高的氦离子辐照通量辐照时,磁化接近面外/面内重取向转变,此时≈100nm尺寸的磁斯格明子得以稳定。正如为具有迷宫畴的超薄膜开发的理论模型所预测的那样,观察到随着氦离子辐照通量增加,斯格明子尺寸减小,而这些磁织构对外加磁场的稳定性增强。