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玻色子离域的偶极莫尔激子。

Bosonic Delocalization of Dipolar Moiré Excitons.

机构信息

Department of Physics, Philipps University, 35037 Marburg, Germany.

出版信息

Nano Lett. 2023 May 24;23(10):4627-4633. doi: 10.1021/acs.nanolett.3c01160. Epub 2023 May 15.

Abstract

In superlattices of twisted semiconductor monolayers, tunable moiré potentials emerge, trapping excitons into periodic arrays. In particular, spatially separated interlayer excitons are subject to a deep potential landscape and they exhibit a permanent dipole providing a unique opportunity to study interacting bosonic lattices. Recent experiments have demonstrated density-dependent transport properties of moiré excitons, which could play a key role for technological applications. However, the intriguing interplay between exciton-exciton interactions and moiré trapping has not been well understood yet. In this work, we develop a microscopic theory of interacting excitons in external potentials allowing us to tackle this highly challenging problem. We find that interactions between moiré excitons lead to a delocalization at intermediate densities, and we show how this transition can be tuned via twist angle and temperature. The delocalization is accompanied by a modification of optical moiré resonances, which gradually merge into a single free exciton peak.

摘要

在扭曲半导体单层的超晶格中,可调谐的莫尔势出现,将激子束缚在周期性的阵列中。特别是,空间分离的层间激子受到深势阱的影响,它们表现出永久偶极矩,为研究相互作用的玻色晶格提供了独特的机会。最近的实验已经证明了莫尔激子的密度依赖性输运性质,这可能在技术应用中发挥关键作用。然而,激子-激子相互作用和莫尔束缚之间的有趣相互作用尚未得到很好的理解。在这项工作中,我们发展了一种在外部势下相互作用激子的微观理论,使我们能够解决这个极具挑战性的问题。我们发现,莫尔激子之间的相互作用导致在中等密度下的离域化,并且我们展示了如何通过扭转角和温度来调节这种转变。离域化伴随着光学莫尔共振的改变,逐渐合并为单个自由激子峰。

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