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用 14MeV D-T 中子诱发 U238 反应中 Xe135m 和 Xe135g 的裂变截面测量。

Fission cross-section measurement for Xe135m and Xe135g in U238 reaction induced by 14MeV D-T neutrons.

机构信息

School of Nuclear Science and Technology, Lanzhou University, Lanzhou, 730000, China.

Institute of Science and Technology of the 404 Company Limited, China National Nuclear Corporation, Jiayuguan, 735100, China.

出版信息

Appl Radiat Isot. 2023 Aug;198:110852. doi: 10.1016/j.apradiso.2023.110852. Epub 2023 May 13.

Abstract

In this work, the independent fission cross-sections of U(n,f)238Xe135g and U(n,f)238Xe135m reactions induced by neutrons with the energies of 14.1 MeV, 14.5 MeV, and 14.7 MeV were measured by activation methods. The neutrons from T(d,n)He4 were used in the experiments and their energies were determined by the ratio of Zr(n,2n)90Zr89 and Nb(n,2n)93Nb92m reaction cross-sections. Aluminum films were chosen as reference samples to measure the neutron fluence relative to the cross section of the Al(n,α)27Na24 reaction. The effect of self-absorption, geometry, and cascade coincidence were also considered during the data analysis. Besides, the increase in the daughter nuclide yield due to the decay of the parent nuclides in the same decay chain was deducted. As a result, the independent fission cross-sections of the U(n,f)238Xe135g reaction are 2.54 ± 0.14 mb, 3.05 ± 0.19 mb and 2.94 ± 0.19 mb, while the cross-sections of U(n,f)238Xe135m reaction are 2.11 ± 0.16 mb, 2.47 ± 0.18 mb and 2.34 ± 0.21 mb for 14.1 MeV, 14.5 MeV and 14.7 MeV neutrons, respectively. This work provides experimental data for the database of nuclear fission reactions.

摘要

在这项工作中,通过激活法测量了能量为 14.1 MeV、14.5 MeV 和 14.7 MeV 的中子诱发的 U(n,f)238Xe135g 和 U(n,f)238Xe135m 反应的独立裂变截面。实验中使用了 T(d,n)He4 产生的中子,其能量通过 Zr(n,2n)90Zr89 和 Nb(n,2n)93Nb92m 反应截面的比值来确定。选择铝膜作为参考样品,以测量相对于 Al(n,α)27Na24 反应截面的中子通量。在数据分析中还考虑了自吸收、几何形状和级联符合的影响。此外,扣除了由于同一条衰变链中的母核衰变而导致子核产额增加的影响。结果,U(n,f)238Xe135g 反应的独立裂变截面分别为 2.54±0.14 mb、3.05±0.19 mb 和 2.94±0.19 mb,而 U(n,f)238Xe135m 反应的截面分别为 2.11±0.16 mb、2.47±0.18 mb 和 2.34±0.21 mb,对于 14.1 MeV、14.5 MeV 和 14.7 MeV 中子。这项工作为核裂变反应数据库提供了实验数据。

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