Han Yafei, Qiao Yujie, Li Zhonglin, Han Xueyan, Wang Qiang, Fang Kaihong, Zhang Shuo
School of Nuclear Science and Technology, Lanzhou University, Lanzhou, 730000, China.
School of Nuclear Science and Technology, Lanzhou University, Lanzhou, 730000, China.
Appl Radiat Isot. 2024 Mar;205:111177. doi: 10.1016/j.apradiso.2024.111177. Epub 2024 Jan 6.
In this study, we conducted measurements of the independent fission cross-sections of U(n, f)Nb, U(n, f)Te reactions and the cumulative cross section of U(n, f)Sb reactions induced by neutron at energies around 14 MeV, i.e., 14.1 ± 0.3, 14.5 ± 0.3 and 14.7 ± 0.3 MeV. The measurement results were obtained by the neutron activation method in combination with off-line γ-ray spectrometry techniques. The neutron flux was monitored on line by the accompanying α-particle from T(d, n)He reaction, and the neutron energies were determined by the cross-section ratio of Zr(n, 2n)Zr to Nb(n, 2n)Nb reactions. The independent fission cross-sections of the fission reactions were obtained by subtracting the influence of precursor nuclei or excited states. The obtained results are as follows: for U(n, f)Nb, the independent cross sections are 1.0 ± 0.89, 0.98 ± 0.85 and 0.78 ± 0.70 mb at the specified neutron energy points. For U(n, f)Te, the independent fission cross-sections are 26.8 ± 2.8, 27.7 ± 2.9 and 20.5 ± 2.3 mb, respectively, at the same neutron energy points. As for (n, f)Sb, the obtained cumulative fission cross-sections are 5.35 ± 0.58, 5.05 ± 0.53 and 4.03 ± 0.44 mb, respectively, at the specified neutron energy points.
在本研究中,我们测量了中子能量在14 MeV左右(即14.1±0.3、14.5±0.3和14.7±0.3 MeV)时U(n, f)Nb、U(n, f)Te反应的独立裂变截面以及U(n, f)Sb反应的累积截面。测量结果通过中子活化法结合离线γ射线能谱技术获得。中子通量通过T(d, n)He反应产生的伴随α粒子进行在线监测,中子能量通过Zr(n, 2n)Zr与Nb(n, 2n)Nb反应的截面比来确定。通过减去前驱核或激发态的影响得到裂变反应的独立裂变截面。获得的结果如下:对于U(n, f)Nb,在指定的中子能量点,独立截面分别为1.0±0.89、0.98±0.85和0.78±0.70 mb。对于U(n, f)Te,在相同的中子能量点,独立裂变截面分别为26.8±2.8、27.7±2.9和20.5±2.3 mb。至于(n, f)Sb,在指定的中子能量点,获得的累积裂变截面分别为5.35±0.58、5.05±0.53和4.03±0.44 mb。