State Key Laboratory of Environmental Aquatic Chemistry, Key Laboratory of Drinking Water Science and Technology, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China; University of Chinese Academy of Sciences, Beijing, 100049, China.
Department of Civil and Environmental Engineering, Imperial College London, South Kensington Campus, London, SW7 2AZ, United Kingdom.
Water Res. 2023 Jul 15;240:120089. doi: 10.1016/j.watres.2023.120089. Epub 2023 May 17.
Drinking water supply in rural areas remains a substantial challenge due to complex natural, technical and economic conditions. To provide safe and affordable drinking water to all, as targeted in the UN Sustainable Development Goals (2030 Agenda), low-cost, efficient water treatment processes suitable for rural areas need to be developed. In this study, a bubbleless aeration BAC (termed ABAC) process is proposed and evaluated, involving the incorporation of a hollow fiber membrane (HFM) assembly within a slow-rate BAC filter, to provide dissolved oxygen (DO) throughout the BAC filter and an increased DOM removal efficiency. The results showed that after a 210-day period of operation, the ABAC increased the DOC removal by 54%, and decreased the disinfection byproduct formation potential (DBPFP) by 41%, compared to a comparable BAC filter without aeration (termed NBAC). The elevated DO (> 4 mg/L) not only reduced secreted extracellular polymer, but also modified the microbial community with a stronger degradation ability. The HFM-based aeration showed comparable performance to 3 mg/L pre-ozonation, and the DOC removal efficiency was four times greater than that of a conventional coagulation process. The proposed ABAC treatment, with its various advantages (e.g., high stability, avoidance of chemicals, ease of operation and maintenance), is well-suited to be integrated as a prefabricated device, for decentralized drinking water systems in rural areas.
由于复杂的自然、技术和经济条件,农村地区的饮用水供应仍然是一个重大挑战。为了按照联合国可持续发展目标(2030 年议程)的目标,为所有人提供安全和负担得起的饮用水,需要开发适合农村地区的低成本、高效的水处理工艺。在这项研究中,提出并评估了一种无泡曝气生物活性炭(ABAC)工艺,该工艺涉及在慢速生物活性炭过滤器中加入中空纤维膜组件,以在整个生物活性炭过滤器中提供溶解氧(DO)并提高 DOM 去除效率。结果表明,与未曝气的可比生物活性炭过滤器(称为 NBAC)相比,ABAC 在 210 天的运行期间将 DOC 去除率提高了 54%,将消毒副产物形成潜力(DBPFP)降低了 41%。升高的 DO(>4mg/L)不仅减少了分泌的胞外聚合物,而且还改变了具有更强降解能力的微生物群落。基于 HFM 的曝气与 3mg/L 预臭氧化具有相当的性能,DOC 去除效率比传统的混凝工艺高四倍。所提出的 ABAC 处理方法具有多种优势(例如,高稳定性、避免使用化学品、易于操作和维护),非常适合作为预制设备集成到农村分散式饮用水系统中。