Alias Nabilah, Ali Umar Akrajas, Sadikin Siti Naqiyah, Ridwan Jaenudin, Hamzah Azrul Azlan, Ali Umar Marjoni Imamora, Ehsan Abang Annuar, Nurdin Muhammad, Zhan Yiqiang
Institute of Microengineering and Nanoelectronics, Universiti Kebangsaan Malaysia, UKM, 43600 Bangi, Selangor, Malaysia.
Department of Physics Education, Faculty of Tarbiyah, Universitas Islam Negeri Mahmud Yunus, Batusangkar 27213, Indonesia.
ACS Omega. 2023 May 18;8(21):18874-18881. doi: 10.1021/acsomega.3c01236. eCollection 2023 May 30.
Perovskite solar cells have emerged as a potential energy alternative due to their low cost of fabrication and high power conversion efficiency. Unfortunately, their poor ambient stability has critically limited their industrialization and application in real environmental conditions. Here, we show that by introducing hexamine molecules into the perovskite lattice, we can enhance the photoactive phase stability, enabling high-performance and air-processable perovskite solar cells. The unencapsulated and freshly prepared perovskite solar cells produce a power conversion efficiency of 16.83% under a 100 mW cm 1.5G solar light simulator and demonstrate high stability properties when being stored for more than 1500 h in humid air with relative humidity ranging from 65 to 90%. We envisage that our findings may revolutionize perovskite solar cell research, pushing the performance and stability to the limit and bringing the perovskite solar cells toward industrialization.
钙钛矿太阳能电池因其制备成本低和功率转换效率高而成为一种潜在的能源替代品。不幸的是,它们较差的环境稳定性严重限制了其工业化进程以及在实际环境条件下的应用。在此,我们表明,通过将六胺分子引入钙钛矿晶格中,可以提高光活性相的稳定性,从而制备出高性能且可通过空气加工的钙钛矿太阳能电池。未封装且刚制备好的钙钛矿太阳能电池在100 mW cm² 1.5G太阳光模拟器下的功率转换效率为16.83%,并且在相对湿度为65%至90%的潮湿空气中储存超过1500小时后仍表现出高稳定性。我们设想,我们的研究结果可能会彻底改变钙钛矿太阳能电池的研究,将其性能和稳定性推向极限,并推动钙钛矿太阳能电池走向工业化。