电化学二氧化碳捕获与浓缩。
Electrochemical Carbon Dioxide Capture and Concentration.
机构信息
Department of Chemistry, University of California, Irvine, California 92697, United States.
Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02142, United States.
出版信息
Chem Rev. 2023 Jul 12;123(13):8069-8098. doi: 10.1021/acs.chemrev.2c00681. Epub 2023 Jun 21.
Electrochemical carbon capture and concentration (eCCC) offers a promising alternative to thermochemical processes as it circumvents the limitations of temperature-driven capture and release. This review will discuss a wide range of eCCC approaches, starting with the first examples reported in the 1960s and 1970s, then transitioning into more recent approaches and future outlooks. For each approach, the achievements in the field, current challenges, and opportunities for improvement will be described. This review is a comprehensive survey of the eCCC field and evaluates the chemical, theoretical, and electrochemical engineering aspects of different methods to aid in the development of modern economical eCCC technologies that can be utilized in large-scale carbon capture and sequestration (CCS) processes.
电化学碳捕获与浓缩（eCCC）为克服温度驱动捕获和释放的局限性提供了一种很有前途的热化学工艺替代方法。本综述将讨论各种 eCCC 方法，从 20 世纪 60 年代和 70 年代首次报道的例子开始，然后转向最近的方法和未来的展望。对于每种方法，将描述该领域的成就、当前的挑战以及改进的机会。本综述是对 eCCC 领域的全面调查，评估了不同方法的化学、理论和电化学工程方面，以帮助开发可用于大规模碳捕获和封存（CCS）过程的现代经济 eCCC 技术。
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