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通过手性超表面中维持的磁偶极子实现非手性分子圆偏振发射的角度控制。

Angular Control of Circularly Polarized Emission from Achiral Molecules via Magnetic Dipoles Sustained in a Chiral Metamirror.

作者信息

Lee Ying-Tsung, Chen Mu-Hsin, Ho Ya-Lun, Wang Zhiyu, Lee Yang-Chun, Delaunay Jean-Jacques

机构信息

School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan.

出版信息

ACS Appl Mater Interfaces. 2023 Aug 2;15(30):36945-36950. doi: 10.1021/acsami.3c05717. Epub 2023 Jul 18.

Abstract

Circularly polarized emission (CPE) plays an important role in the designs of advanced displays and photonic integrated circuits. Unfortunately, the control of CPE handedness is limited by the chiral metasurfaces employed to emit chiral light. Particularly, the switching of the handedness with chiral metasurfaces relies on flipping the metasurfaces, which adds some constraints to practical applications. Herein, we propose an angle-sensitive chiral metamirror with Mie resonators to realize handedness switching. The Mie resonator supports a magnetic dipole having large field enhancement. This chiral metamirror is applied to excite CPEs with opposite handedness at emission angles within 10°. In contrast to the conventional methods, this work proposes a more efficient approach to manipulate the handedness of CPE.

摘要

圆偏振发射(CPE)在先进显示器和光子集成电路的设计中起着重要作用。不幸的是,CPE手性的控制受到用于发射手性光的手性超表面的限制。特别是,利用手性超表面进行手性切换依赖于翻转超表面,这给实际应用带来了一些限制。在此,我们提出一种带有米氏谐振器的角度敏感型手性超表面镜来实现手性切换。米氏谐振器支持具有大场增强的磁偶极子。这种手性超表面镜用于在10°以内的发射角激发具有相反手性的CPE。与传统方法相比,这项工作提出了一种更有效的方法来操纵CPE的手性。

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