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用于核能与医学应用的TeO/WO/KO复合玻璃系统的力学弹性性能及辐射衰减效率

Mechanic-elastic properties and radiation attenuation efficiency of TeO/WO/KO composite glass systems for nuclear and medical application.

作者信息

Alsaif Norah A M, Khattari Z Y, Zakaly Hesham M H, Rammah Y S, Ene Antoaneta, Al-Buriahi M S

机构信息

Department of Physics, College of Science, Princess Nourah Bint Abdulrahman University, P.O. Box 84428, Riyadh, 11671, Saudi Arabia.

Department of Physics, Faculty of Science, The Hashemite University, P. O. Box 330127, Zarqa, 13133, Jordan.

出版信息

Heliyon. 2023 Aug 4;9(8):e18912. doi: 10.1016/j.heliyon.2023.e18912. eCollection 2023 Aug.

Abstract

WO effects on neutron and ionizing radiation defending factors of ternary tellurite-based glass blocks with molecular formula 80TeO -(20-x)WO - xKO; x = 0-20 mol% (denoted as TKW-glass) has been reported via Phy-X theoretical calculations and Geant4 simulation code. Correlations between shielding factors and kinetics properties of the investigated glasses at different photon energy have been examined. The highest values of mass (MAC) attenuation coefficient were noted at 15 keV of the examined TKW-glass materials with the values of 38.408, 44.388, 49.855, 54.872, 59.492 cm/g for TKW-0, TKW-5, TKW-10, TKW-15, and TKW-20, respectively. Generally, these values of the TKW-glasses obey the sequence: (TKW-0)< (TKW-5) < (TKW-10) < (TKW-15) < (TKW-20). The highest mean free path (MFP) values of TKW-glasses were registered at 15 MeV with the values of 6.101, 5.591, 5.097, 4.647, and 4.302 cm for TKW-0, TKW-5, TKW-10, TKW-15, and TKW-20, respectively. The two parameters half value layer (HVL) and MFP follow the pattern: (TKW-0) > (TKW-5) > (TKW-10) > (TKW-15) > (TKW-20). The maximum values of effective atomic number (EAN) took place at gamma energy of 15 keV corresponding to 44.35, 48.86, 52.63, 55.83, and 58.58 for TKW-0, TKW-5, TKW-10, TKW-15, and TKW-20, respectively. The trend of the buildup factors was similar for all of the glass specimens. The fast neutron removal cross-section () enhanced as WO content increased in the specimens. Thus, the peaked value of is 0.1059 cm was noted in the TKW-20 sample. Mechanical properties, neutron and γ-rays protection parameters were observed to improve with enhanced WO mol% in the TKW-glasses. The current results bear their utilization for neutron and gamma protection purposes.

摘要

通过Phy-X理论计算和Geant4模拟代码,报道了分子式为80TeO₂-(20-x)WO₃ - xK₂O;x = 0-20 mol%(表示为TKW-玻璃)的三元碲酸盐基玻璃块对中子和电离辐射防护因子的影响。研究了不同光子能量下被研究玻璃的屏蔽因子与动力学性质之间的相关性。在所研究的TKW-玻璃材料中,在15 keV时质量(MAC)衰减系数达到最高值,TKW-0、TKW-5、TKW-10、TKW-15和TKW-20的MAC值分别为38.408、44.388、49.855、54.872、59.492 cm/g。一般来说,TKW-玻璃的这些值遵循以下顺序:(TKW-0) < (TKW-5) < (TKW-10) < (TKW-15) < (TKW-20)。TKW-玻璃的最高平均自由程(MFP)值在15 MeV时记录,TKW-0、TKW-5、TKW-10、TKW-15和TKW-20的MFP值分别为6.101、5.591、5.097、4.647和4.302 cm。半值层(HVL)和MFP这两个参数遵循以下模式:(TKW-0) > (TKW-5) > (TKW-10) > (TKW-15) > (TKW-20)。有效原子序数(EAN)的最大值出现在15 keV的伽马能量处,TKW-0、TKW-5、TKW-10、TKW-15和TKW-20对应的EAN值分别为44.35、48.86、52.63、55.83和58.58。所有玻璃样品的积累因子趋势相似。随着样品中WO含量的增加,快中子去除截面()增大。因此,在TKW-20样品中观察到的峰值为0.1059 cm。随着TKW-玻璃中WO摩尔百分比的增加,观察到机械性能、中子和γ射线防护参数得到改善。目前的结果表明它们可用于中子和伽马防护目的。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/862e/10432205/0036f52ab035/gr1.jpg

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