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氧化钠改性碲酸盐玻璃体系的辐射屏蔽性能评估

Evaluation of the Radiation Shielding Properties of a Tellurite Glass System Modified with Sodium Oxide.

作者信息

Hussein Khalid I, Alqahtani Mohammed S, Meshawi Arwa A, Alzahrani Khloud J, Zahran Heba Y, Alshehri Ali M, Yahia Ibrahim S, Reben Manuela, Yousef El Sayed

机构信息

Department of Radiological Sciences, College of Applied Medical Sciences, King Khalid University, Abha 61421, Saudi Arabia.

Department of Medical Physics and Instrumentation, National Cancer Institute, University of Gezira, Wad Medani 2667, Sudan.

出版信息

Materials (Basel). 2022 Apr 27;15(9):3172. doi: 10.3390/ma15093172.

Abstract

In this study, the X-ray and gamma attenuation characteristics and optical properties of a synthesized tellurite-phosphate-sodium oxide glass system with a composition of (85 - x)TeO-10PO-xNaO mol% (where x = 15, 20, and 25) were evaluated. The glass systems we re fabricated by our research group using quenching melt fabrication. The shielding parameters of as-synthesized systems, such as the mass attenuation coefficient (MAC), linear attenuation coefficient (LAC), effective atomic number (Z), half-value layer (HVL), tenth value layer (TVL), mean free path (MFP), and effective electron density (N) in a wide energy range between 15 keV and 15 MeV, were estimated using well-known PHY-X/PSD software and recently developed MIKE software. Herein, the optical parameters of prepared glasses, such as molar volume (V), oxygen molar volume (V), oxygen packing density (OPD), molar polarizability (αm), molar refractivity (R), reflection loss (R), and metallization (M), were estimated using MIKE software. Furthermore, the shielding performance of the prepared glasses was compared with that of commonly used standard glass shielding materials. The results show that the incorporation of sodium oxide into the matrix TeO/PO with an optimum concentration can yield a glass system with good shielding performance as well as good optical and physical properties, especially at low photon energy.

摘要

在本研究中,对组成为(85 - x)TeO₂-10P₂O₅-xNa₂O摩尔百分比(其中x = 15、20和25)的合成碲酸盐-磷酸盐-氧化钠玻璃体系的X射线和γ射线衰减特性以及光学性质进行了评估。这些玻璃体系由我们的研究小组采用骤冷熔体法制备而成。使用著名的PHY-X/PSD软件和最近开发的MIKE软件,估算了合成体系在15 keV至15 MeV的宽能量范围内的屏蔽参数,如质量衰减系数(MAC)、线性衰减系数(LAC)、有效原子序数(Z)、半价层(HVL)、十分之一值层(TVL)、平均自由程(MFP)和有效电子密度(N)。在此,使用MIKE软件估算了所制备玻璃的光学参数,如摩尔体积(V)、氧摩尔体积(V)、氧堆积密度(OPD)、摩尔极化率(αm)、摩尔折射率(R)、反射损失(R)和金属化率(M)。此外,将所制备玻璃的屏蔽性能与常用的标准玻璃屏蔽材料的屏蔽性能进行了比较。结果表明,以最佳浓度将氧化钠掺入基体TeO₂/P₂O₅中,可得到一种具有良好屏蔽性能以及良好光学和物理性质的玻璃体系,尤其是在低光子能量下。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/5ffd/9100053/099434c083a7/materials-15-03172-g001.jpg

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