Rubinsztajn Slawomir, Chojnowski Julian, Mizerska Urszula
Centre of Molecular and Macromolecular Studies of Polish Academy of Sciences, Sienkiewicza 112, 90-636 Lodz, Poland.
Molecules. 2023 Aug 8;28(16):5941. doi: 10.3390/molecules28165941.
Tris(pentafluorophenyl)borane (TPFPB) is a unique Lewis acid that catalyzes the condensation between hydrosilanes (Si-H) and alkoxysilanes (Si-OR), leading to the formation of siloxane bonds (Si-OSi) with the release of hydrocarbon (R-H) as a byproduct-the so-called Piers-Rubinsztajn reaction. The analogous reactions of hydrosilanes with silanols (Si-OH), alcohols (R-OH), ethers (R-OR') or water in the presence of TPFPB leads to the formation of a siloxane bond, alkoxysilane (Si-OR or Si-OR') or silanol (Si-OH), respectively. The above processes, often referred to as Piers-Rubinsztajn reactions, provide new synthetic tools for the controlled synthesis of siloxane materials under mild conditions with high yields. The common feature of these reactions is the TPFPB-mediated hydride transfer from silicon to carbon or hydrogen. This review presents a summary of 20 years of research efforts related to this field, with a focus on new synthetic methodologies leading to numerous previously difficult to synthesize well-defined siloxane oligomers, polymers and copolymers of a complex structure and potential applications of these new materials. In addition, the mechanistic aspects of the recently discovered reactions involving hydride transfer from silicon to silicon are discussed in more detail.
三(五氟苯基)硼烷(TPFPB)是一种独特的路易斯酸,它催化氢硅烷(Si-H)与烷氧基硅烷(Si-OR)之间的缩合反应,生成硅氧烷键(Si-OSi),并副产烃类(R-H)——即所谓的皮尔斯-鲁宾斯泰因反应。在TPFPB存在下,氢硅烷与硅醇(Si-OH)、醇类(R-OH)、醚类(R-OR')或水的类似反应分别生成硅氧烷键、烷氧基硅烷(Si-OR或Si-OR')或硅醇(Si-OH)。上述过程通常称为皮尔斯-鲁宾斯泰因反应,为在温和条件下高产率地可控合成硅氧烷材料提供了新的合成工具。这些反应的共同特点是TPFPB介导氢从硅转移至碳或氢。本综述总结了该领域20年的研究成果,重点介绍了新的合成方法,这些方法可合成许多以前难以合成的结构复杂的、定义明确的硅氧烷低聚物、聚合物和共聚物,以及这些新材料的潜在应用。此外,还更详细地讨论了最近发现的涉及氢从硅转移至硅的反应的机理方面。