Saint-Petersburg Research Institute of Radiation Hygiene after Professor P.V. Ramzaev, 8 Mira Str., 197101, Saint-Petersburg, Russian Federation.
J Environ Radioact. 2023 Dec;270:107283. doi: 10.1016/j.jenvrad.2023.107283. Epub 2023 Aug 25.
This study evaluates the air kerma rate in radioactively contaminated forests. The air kerma rates created by plane sources of monoenergetic photons in the energy range 0.02-3 MeV located at different depths in soil up to 50 g cm and at different heights in the forest medium from 0.05 to 50 m were calculated using numeric solution of the transport (Boltzmann) equation. To simplify the practical use of the results obtained by solving the Boltzmann equation, the study additionally includes approximation formulae for calculating air kerma rate separately from contaminated soil, crowns and trunks of trees in a forest ecosystem for 20 radionuclides - fission products that significantly contribute to the external dose. Biomaterial of trunks and crowns was modeled as uniformly distributed in corresponding layers and homogeneously mixed with air. Different distributions of radionuclides in soil were considered including plane source located at different depths, exponential and uniform distribution. Based on the results, the effect of forest biomass presence as an absorbing and scattering medium on the air kerma rate at 1 m above soil was evaluated. The estimated relative difference in air kerma rate at 1 m above soil in the forest medium and in free air for monoenergetic photon sources with energies 0.1 MeV, 0.66 MeV and 3 MeV did not correlate significantly with the energy of photons. Its maximum value in forest medium with biomass density of 5 kg m was 15-20% for the source at soil depth ∼0.3 g cm, decreasing to less than 5% when it is at soil depth greater than 7 g cm. An example calculation of the air kerma rate dynamics is presented for the initial period after radioactive fallout considering weathering processes (rainfall and wind action) that contribute to the transfer of activity from the canopies to the forest floor. The differences in air kerma rate values, as an integral characteristic of the gamma radiation field from a radioactive cloud in the forest and in the open area, were evaluated.
本研究评估了放射性污染森林中的空气比释动能率。使用数值解方法,对位于土壤中不同深度(0.02-3 MeV 能量范围内)的单能光子平面源在森林介质中不同高度(0.05-50 m)产生的空气比释动能率进行了计算。为了简化通过求解 Boltzmann 方程获得的结果的实际应用,该研究还包含了针对 20 种放射性核素(对外部剂量有重要贡献的裂变产物)的污染土壤、树冠和树干分别计算空气比释动能率的近似公式。树木的生物量被建模为均匀分布在相应的层中,并与空气均匀混合。考虑了土壤中不同的放射性核素分布,包括位于不同深度的平面源、指数分布和均匀分布。基于这些结果,评估了森林生物量作为吸收和散射介质对土壤上方 1 m 处空气比释动能率的影响。对于能量为 0.1 MeV、0.66 MeV 和 3 MeV 的单能光子源,在森林介质中和自由空气中 1 m 处的空气比释动能率的估计相对差异与光子能量没有显著相关性。在生物量密度为 5 kg m 的森林介质中,当源位于土壤深度约 0.3 g cm 时,最大差异为 15-20%,当源位于土壤深度大于 7 g cm 时,最大差异减小到小于 5%。本研究还展示了一个放射性沉降后初始时期的空气比释动能率动态的示例计算,考虑了风化过程(降雨和风的作用),这些过程有助于将放射性核素从树冠转移到森林地面。评估了放射性云在森林和开阔区域中的伽马辐射场的空气比释动能率值作为一个整体特征的差异。