Silkin Vyacheslav M, Drechsler Stefan-Ludwig, Efremov Dmitry V
Donostia International Physics Center (DIPC), 20018 San Sebastián/Donostia, Basque Country, Spain.
Departamento de Polímeros y Materiales Avanzados: Física, Química y Tecnología, Facultad de Ciencias Químicas, Universidad del País Vasco UPV/EHU, 20080 San Sebastián/Donostia, Basque Country, Spain.
J Phys Chem Lett. 2023 Sep 14;14(36):8060-8068. doi: 10.1021/acs.jpclett.3c01871. Epub 2023 Sep 1.
Despite decades of intensive experimental and theoretical efforts, the physics of cuprate high-temperature superconductors in general, and, in particular, their normal state, is still under debate. Here, we report our investigation of low-energy charge excitations in the normal state. We find that the peculiarities of the electronic band structure at low energies have a profound impact on the nature of the intraband collective modes. It gives rise to a new kind of mode with huge intensity and non-Lorentzian spectral function in addition to well-known collective excitations like conventional plasmons and spin fluctuation. We predict two such modes with maximal spectral weight in the nodal and antinodal directions. Additionally, we found a long-living quasi-one-dimensional plasmon becoming an intense soft mode over an extended momentum range along the antinodal direction. These modes might explain some of the resonant inelastic X-ray scattering spectroscopy data.
尽管经过了数十年密集的实验和理论研究,但铜酸盐高温超导体的物理学,尤其是其正常态,仍存在争议。在此,我们报告我们对正常态低能电荷激发的研究。我们发现低能电子能带结构的特性对带内集体模式的性质有深远影响。除了传统等离子体激元和自旋涨落等已知的集体激发外,它还产生了一种具有巨大强度和非洛伦兹谱函数的新型模式。我们预测在节点和反节点方向有两种具有最大谱权重的此类模式。此外,我们发现一种寿命较长的准一维等离子体激元在沿反节点方向的扩展动量范围内变成一种强烈的软模式。这些模式可能解释一些共振非弹性X射线散射光谱数据。