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关于从景观水中去除新兴污染物的改良浮式光催化剂的批判性回顾:问题、方法和机制。

Critical review on modified floating photocatalysts for emerging contaminants removal from landscape water: problems, methods and mechanism.

机构信息

College of Safety and Environmental Engineering, Shandong University of Science and Technology, Qingdao, China.

China Testing & Certification International Group Qingdao Jingcheng Testing Co., Ltd., Qingdao, 266426, China.

出版信息

Chemosphere. 2023 Nov;341:140043. doi: 10.1016/j.chemosphere.2023.140043. Epub 2023 Sep 1.

Abstract

Due to the disorderly discharge in modern production and daily life of people, emerging contaminants(ECs) began to appear in landscape water, and have become a key public concern. Because of the unique characteristics of landscape water, it is difficult to efficiently remove ECs either by natural purification or by traditional large-scale sewage treatment facilities. The ideal purification method is to remove them while maintaining a beautiful environment. Possessing the feature of low-density, floating photocatalysts could harvest sufficient light on the surface of the water for photocatalytic degradation, which may be an important supplement for ECs treatment in landscape water. This paper gave a review related to floating photocatalysts and proposed an idea of combining floating photocatalysts to construct bionic photocatalytic materials for contaminative landscape water treatment. Six types of common floating substrates and corresponding applications for floating photocatalysts were concluded in this paper, and the main problem leading to the low efficiency of photocatalysts and three corresponding three improvement strategies were discussed. Besides, the modification mechanisms of photocatalysts were discussed thoroughly. On this basis, the engineering application prospects of bionic photocatalytic materials were proposed to remove ECs in landscape water.

摘要

由于现代生产和日常生活中的无序排放,新兴污染物(ECs)开始出现在景观水中,成为公众关注的焦点。由于景观水的独特性质,无论是通过自然净化还是通过传统的大型污水处理设施,都很难有效地去除 ECs。理想的净化方法是在保持优美环境的同时去除它们。具有低密度、漂浮特性的光催化剂可以在水面上收集足够的光进行光催化降解,这可能是景观水 ECs 处理的重要补充。本文综述了漂浮光催化剂,并提出了将漂浮光催化剂与仿生光催化材料相结合,用于处理污染景观水的思路。本文总结了六种常见的漂浮基质及其相应的漂浮光催化剂应用,并讨论了导致光催化剂效率低下的主要问题及三种相应的改进策略。此外,还深入探讨了光催化剂的改性机制。在此基础上,提出了仿生光催化材料去除景观水中 ECs 的工程应用前景。

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