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基于透明二氧化硅纳米腔的防水亚波长钙钛矿激光发射

Water-Resistant Subwavelength Perovskite Lasing from Transparent Silica-Based Nanocavity.

作者信息

Huang Sihao, Shen Zixi, Liao Yang, Liu Zhengzheng, Hu Zhiping, Li Qian, Zhang Zeyu, Dong Siyu, Luo Jiajun, Du Juan, Tang Jiang, Leng Yuxin

机构信息

State Key Laboratory of High Field Laser Physics and CAS Center for Excellence in Ultra-Intense Laser Science, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, 201800, China.

Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, 100049, China.

出版信息

Adv Mater. 2023 Dec;35(52):e2306102. doi: 10.1002/adma.202306102. Epub 2023 Nov 20.

DOI:10.1002/adma.202306102
PMID:37669761
Abstract

Great research efforts are devoted to exploring the miniaturization of chip-scale coherent light sources possessing excellent lasing performance. Despite the indispensable role in Si photonics, SiO is generally considered not contributing to the starting up and operation of integrated lasers. Here, this work demonstrates an extraordinary-performance subwavelength-scale perovskite vertical cavity laser with all-transparent SiO cavity, whose cavity is ultra-simple and composed of only two parallel SiO plates. By introducing a ligand-assisted thermally co-evaporation strategy, highly luminescent perovskite film with high reproducibility and excellent optical gain is grown directly on SiO . Benefitting from their high-refractive-index contrast, low-threshold, high-quality factor, and single-mode lasing is achieved in subwavelength range of ≈120 nm, and verified by long-range coherence distance (115.6 µm) and high linear polarization degree (82%). More importantly, the subwavelength perovskite laser device could operate in water for 20 days without any observable degradation, exhibiting ultra-stable water-resistant performance. These findings would provide a simple but robust and reliable strategy for the miniaturized on-chip lasers compatible with Si photonics.

摘要

大量的研究工作致力于探索具有优异激光性能的芯片级相干光源的小型化。尽管SiO在硅光子学中起着不可或缺的作用,但通常认为它对集成激光器的启动和运行没有贡献。在此,这项工作展示了一种具有全透明SiO腔的超高性能亚波长尺度钙钛矿垂直腔激光器,其腔非常简单,仅由两个平行的SiO板组成。通过引入配体辅助热共蒸发策略,在SiO上直接生长出具有高重现性和优异光学增益的高发光钙钛矿薄膜。受益于它们的高折射率对比度,在约120nm的亚波长范围内实现了低阈值、高品质因数和单模激光发射,并通过长程相干长度(115.6μm)和高线性偏振度(82%)得到验证。更重要的是,亚波长钙钛矿激光器件可以在水中运行20天而没有任何可观察到的降解,表现出超稳定的防水性能。这些发现将为与硅光子学兼容的小型化片上激光器提供一种简单但强大且可靠的策略。

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Water-Resistant Subwavelength Perovskite Lasing from Transparent Silica-Based Nanocavity.基于透明二氧化硅纳米腔的防水亚波长钙钛矿激光发射
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Facet-selective growth of halide perovskite/2D semiconductor van der Waals heterostructures for improved optical gain and lasing.
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